Abstract

Solid-state single-photon sources (SPS) based on quantum dots as well as color centers in diamonds and silicon-carbide have promise for application in emerging quantum technologies. Many of these technologies, however, demand photon rates in the GHz range, thereby hindering the use of these SPS, for which the maximum observed count rates are limited to a few tens of MHz. Here we first study the performance of hyperbolic metamaterial-based 5-layered metal–dielectric resonator antenna structures with metallic as well as hybrid metal–dielectric antennas in the wavelength range of 600 to 1000 nm. The performance of these resonator-antenna structures was analyzed for the Purcell enhancement, quantum efficiency (QE), collection efficiency (CE), and normalized collected photon counts (NCPC). The hybrid metal–dielectric antenna helps in providing the directivity to the dipole emission, thereby significantly improving the collection efficiency. We then present the novel design of a 5-layered metal–dielectric pillar resonator. This resonator structure with a metallic cylindrical antenna over the top showed significantly large fluorescence enhancement values. The Purcell factor was observed to reach close to 1600 at 680 nm corresponding to the central peak of the nitrogen vacancy center spectrum. The NCPC value reached close to 550 at 680 nm. The maximum CE from the structure was observed to be around 60%, with the maximum QE reaching close to 80%. With the above performance, the detected photon count rates for a solid-state SPS is expected to be well into the GHz range. Our designs show a state-of-the-art improvement in the antenna performance for SPS with properties very close to a practical SPS.

© 2020 Optical Society of America

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References

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2020 (1)

A. Kala, F. A. Inam, S. Biehs, P. Vaity, and V. G. Achanta, “Hyperbolic metamaterial with quantum dots for enhanced emission and collection efficiencies,” Adv. Opt. Mater. 8, 2000368 (2020).
[Crossref]

2019 (1)

S. Castelletto, A. S. Al Atem, F. A. Inam, H. J. von Bardeleben, S. Hameau, A. F. Almutairi, G. Guillot, S. Sato, A. Boretti, and J. M. Bluet, “Deterministic placement of ultra-bright near-infrared color centers in arrays of silicon carbide micropillars,” Beilstein J. Nanotechnol. 10, 2383–2395 (2019).
[Crossref]

2018 (4)

F. A. Inam, N. Ahmed, M. J. Steel, and S. Castelletto, “Hyperbolic metamaterial resonator–antenna scheme for large, broadband emission enhancement and single-photon collection,” J. Opt. Soc. Am. B 35, 2153–2162 (2018).
[Crossref]

S. I. Bogdanov, M. Y. Shalaginov, A. S. Lagutchev, C.-C. Chiang, D. Shah, A. S. Baburin, I. A. Ryzhikov, I. A. Rodionov, A. V. Kildishev, A. Boltasseva, and V. M. Shalaev, “Ultrabright room-temperature sub-nanosecond emission from single nitrogen-vacancy centers coupled to nanopatch antennas,” Nano Lett. 18, 4837–4844 (2018).
[Crossref]

A. Karamlou, M. E. Trusheim, and D. Englund, “Metal-dielectric antennas for efficient photon collection from diamond color centers,” Opt. Express 26, 3341–3352 (2018).
[Crossref]

N. H. Wan, B. J. Shields, D. Kim, S. Mouradian, B. Lienhard, M. Walsh, H. Bakhru, T. Schröder, and D. Englund, “Efficient extraction of light from a nitrogen-vacancy center in a diamond parabolic reflector,” Nano Lett. 18, 2787–2793 (2018).
[Crossref]

2017 (4)

A. Lohrmann, B. C. Johnson, J. C. McCallum, and S. Castelletto, “A review on single photon sources in silicon carbide,” Rep. Prog. Phys. 80, 034502 (2017).
[Crossref]

A. F. Koenderink, “Single-photon nanoantennas,” ACS Photon. 4, 710–722 (2017).
[Crossref]

S. Axelrod, M. K. Dezfouli, H. M. K. Wong, A. S. Helmy, and S. Hughes, “Hyperbolic metamaterial nanoresonators make poor single-photon sources,” Phys. Rev. B 95, 155424 (2017).
[Crossref]

M. Radulaski, M. Widmann, M. Niethammer, J. L. Zhang, S.-Y. Lee, T. Rendler, K. G. Lagoudakis, N. T. Son, E. Janzén, T. Ohshima, J. Wrachtrup, and J. Vučković, “Scalable quantum photonics with single color centers in silicon carbide,” Nano Lett. 17, 1782–1786 (2017).
[Crossref]

2016 (3)

T. B. Hoang, G. M. Akselrod, and M. H. Mikkelsen, “Ultrafast room-temperature single photon emission from quantum dots coupled to plasmonic nanocavities,” Nano Lett. 16, 270–275 (2016).
[Crossref]

T. Li and J. B. Khurgin, “Hyperbolic metamaterials: beyond the effective medium theory,” Optica 3, 1388–1396 (2016).
[Crossref]

I. Aharonovich, D. Englund, and M. Toth, “Solid-state single-photon emitters,” Nat. Photonics 10, 631–641 (2016).
[Crossref]

2015 (6)

T. T. Tran, K. Bray, M. J. Ford, M. Toth, and I. Aharonovich, “Quantum emission from hexagonal boron nitride monolayers,” Nat. Nanotechnol. 11, 37–41 (2015).
[Crossref]

M. Pelton, “Modified spontaneous emission in nanophotonic structures,” Nat. Photonics 9, 427–435 (2015).
[Crossref]

T. Galfsky, H. N. S. Krishnamoorthy, W. Newman, E. E. Narimanov, Z. Jacob, and V. M. Menon, “Active hyperbolic metamaterials: enhanced spontaneous emission and light extraction,” Optica 2, 62–65 (2015).
[Crossref]

M. Y. Shalaginov, V. V. Vorobyov, J. Liu, M. Ferrera, A. V. Akimov, A. Lagutchev, A. N. Smolyaninov, V. V. Klimov, J. Irudayaraj, A. V. Kildishev, A. Boltasseva, and V. M. Shalaev, “Enhancement of single-photon emission from nitrogen-vacancy centers with TiN/(Al,Sc)N hyperbolic metamaterial,” Laser Photon. Rev. 9, 120–127 (2015).
[Crossref]

P.-B. Li, Y.-C. Liu, S.-Y. Gao, Z.-L. Xiang, P. Rabl, Y.-F. Xiao, and F.-L. Li, “Hybrid quantum device based on NV centers in diamond nanomechanical resonators plus superconducting waveguide cavities,” Phys. Rev. Appl. 4, 044003 (2015).
[Crossref]

L. Li, E. H. Chen, J. Zheng, S. L. Mouradian, F. Dolde, T. Schröder, S. Karaveli, M. L. Markham, D. J. Twitchen, and D. Englund, “Efficient photon collection from a nitrogen vacancy center in a circular bullseye grating,” Nano Lett. 15, 1493–1497 (2015).
[Crossref]

2014 (5)

L. Ferrari, D. Lu, D. Lepage, and Z. Liu, “Enhanced spontaneous emission inside hyperbolic metamaterials,” Opt. Express 22, 4301–4306 (2014).
[Crossref]

O. D. Miller, S. G. Johnson, and A. W. Rodriguez, “Effectiveness of thin films in lieu of hyperbolic metamaterials in the near field,” Phys. Rev. Lett. 112, 157402 (2014).
[Crossref]

W. Pfaff, B. J. Hensen, H. Bernien, S. B. Van Dam, M. S. Blok, T. H. Taminiau, M. J. Tiggelman, R. N. Schouten, M. Markham, D. J. Twitchen, and R. Hanson, “Unconditional quantum teleportation between distant solid-state quantum bits,” Science 345, 532–535 (2014).
[Crossref]

G. M. Akselrod, C. Argyropoulos, T. B. Hoang, C. Ciracì, C. Fang, J. Huang, D. R. Smith, and M. H. Mikkelsen, “Probing the mechanisms of large Purcell enhancement in plasmonic nanoantennas,” Nat. Photonics 8, 835–840 (2014).
[Crossref]

F. Bigourdan, F. Marquier, J.-P. Hugonin, and J.-J. Greffet, “Design of highly efficient metallo-dielectric patch antennas for single-photon emission,” Opt. Express 22, 2337–2347 (2014).
[Crossref]

2013 (6)

F. A. Inam, M. D. W. Grogan, M. Rollings, T. Gaebel, J. M. Say, C. Bradac, T. A. Birks, W. J. Wadsworth, S. Castelletto, J. R. Rabeau, and M. J. Steel, “Emission and nonradiative decay of nanodiamond NV centers in a low refractive index environment,” ACS Nano 7, 3833–3843 (2013).
[Crossref]

A. Mohtashami and A. Femius Koenderink, “Suitability of nano-diamond nitrogen–vacancy centers for spontaneous emission control experiments,” New J. Phys. 15, 043017 (2013).
[Crossref]

F. A. Inam, A. M. Edmonds, M. J. Steel, and S. Castelletto, “Tracking emission rate dynamics of nitrogen vacancy centers in nano-diamonds,” Appl. Phys. Lett. 102, 253109 (2013).
[Crossref]

W. D. Newman, C. L. Cortes, and Z. Jacob, “Enhanced and directional single-photon emission in hyperbolic metamaterials,” J. Opt. Soc. Am. B 30, 766 (2013).
[Crossref]

A. Poddubny, I. Iorsh, P. Belov, and Y. Kivshar, “Hyperbolic metamaterials,” Nat. Photonics 7, 948–957 (2013).
[Crossref]

M. Y. Shalaginov, S. Ishii, J. Liu, J. Liu, J. Irudayaraj, A. Lagutchev, A. V. Kildishev, and V. M. Shalaev, “Broadband enhancement of spontaneous emission from nitrogen-vacancy centers in nano-diamonds by hyperbolic metamaterials,” Appl. Phys. Lett. 102, 173114 (2013).
[Crossref]

2012 (4)

D. H. Hwang, J. H. Ahn, K. N. Hui, K. S. Hui, and Y. G. Son, “Structural and optical properties of ZnS thin films deposited by RF magnetron sputtering,” Nanoscale Res. Lett. 7, 26 (2012).
[Crossref]

H. N. S. Krishnamoorthy, Z. Jacob, E. Narimanov, I. Kretzschmar, and V. M. Menon, “Topological transitions in metamaterials,” Science 336, 205–209 (2012).
[Crossref]

S. Buckley, K. Rivoire, and J. Vučković, “Engineered quantum dot single-photon sources,” Rep. Prog. Phys. 75, 126503 (2012).
[Crossref]

S. Bounouar, M. Elouneg-Jamroz, M. den Hertog, C. Morchutt, E. Bellet-Amalric, R. André, C. Bougerol, Y. Genuist, J.-P. Poizat, S. Tatarenko, and K. Kheng, “Ultrafast room temperature single-photon source from nanowire-quantum dots,” Nano Lett. 12, 2977–2981 (2012).
[Crossref]

2011 (4)

I. Aharonovich, S. Castelletto, D. A. Simpson, C.-H. Su, A. D. Greentree, and S. Prawer, “Diamond-based single-photon emitters,” Rep. Prog. Phys. 74, 076501 (2011).
[Crossref]

S. Castelletto, J. P. Harrison, L. Marseglia, A. C. Stanley-Clarke, B. C. Gibson, B. A. Fairchild, J. P. Hadden, Y.-L. D. Ho, M. P. Hiscocks, K. Ganesan, S. T. Huntington, F. Ladouceur, A. D. Greentree, S. Prawer, J. L. O’Brien, and J. G. Rarity, “Diamond-based structures to collect and guide light,” New J. Phys. 13, 025020 (2011).
[Crossref]

F. A. Inam, T. Gaebel, C. Bradac, L. Stewart, M. J. Withford, J. M. Dawes, J. R. Rabeau, and M. J. Steel, “Modification of spontaneous emission from nano-diamond colour centers on a structured surface,” New J. Phys. 13, 073012 (2011).
[Crossref]

J. I. Larruquert, A. P. Pérez-Marín, S. García-Cortés, L. Rodríguez-de Marcos, J. A. Aznárez, and J. A. Méndez, “Self-consistent optical constants of SiC thin films,” J. Opt. Soc. Am. A 28, 2340–2345 (2011).
[Crossref]

2010 (3)

T. M. Babinec, B. J. M. Hausmann, M. Khan, Y. Zhang, J. R. Maze, P. R. Hemmer, and M. Lončar, “A diamond nanowire single-photon source,” Nat. Nanotechnol. 5, 195–199 (2010).
[Crossref]

M. G. Blaber, M. D. Arnold, and M. J. Ford, “A review of the optical properties of alloys and intermetallics for plasmonics,” J. Phys. Condens. Matter 22, 143201 (2010).
[Crossref]

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H. Chew, “Radiation and lifetimes of atoms inside dielectric particles,” Phys. Rev. A 38, 3410–3416 (1988).
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J. R. Rabeau, Y. L. Chin, S. Prawer, F. Jelezko, T. Gaebel, and J. Wrachtrup, “Fabrication of single nickel-nitrogen defects in diamond by chemical vapor deposition,” Appl. Phys. Lett. 86, 131926 (2005).
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G. M. Akselrod, C. Argyropoulos, T. B. Hoang, C. Ciracì, C. Fang, J. Huang, D. R. Smith, and M. H. Mikkelsen, “Probing the mechanisms of large Purcell enhancement in plasmonic nanoantennas,” Nat. Photonics 8, 835–840 (2014).
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Dawes, J. M.

F. A. Inam, T. Gaebel, C. Bradac, L. Stewart, M. J. Withford, J. M. Dawes, J. R. Rabeau, and M. J. Steel, “Modification of spontaneous emission from nano-diamond colour centers on a structured surface,” New J. Phys. 13, 073012 (2011).
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S. Bounouar, M. Elouneg-Jamroz, M. den Hertog, C. Morchutt, E. Bellet-Amalric, R. André, C. Bougerol, Y. Genuist, J.-P. Poizat, S. Tatarenko, and K. Kheng, “Ultrafast room temperature single-photon source from nanowire-quantum dots,” Nano Lett. 12, 2977–2981 (2012).
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S. Axelrod, M. K. Dezfouli, H. M. K. Wong, A. S. Helmy, and S. Hughes, “Hyperbolic metamaterial nanoresonators make poor single-photon sources,” Phys. Rev. B 95, 155424 (2017).
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L. Li, E. H. Chen, J. Zheng, S. L. Mouradian, F. Dolde, T. Schröder, S. Karaveli, M. L. Markham, D. J. Twitchen, and D. Englund, “Efficient photon collection from a nitrogen vacancy center in a circular bullseye grating,” Nano Lett. 15, 1493–1497 (2015).
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F. A. Inam, A. M. Edmonds, M. J. Steel, and S. Castelletto, “Tracking emission rate dynamics of nitrogen vacancy centers in nano-diamonds,” Appl. Phys. Lett. 102, 253109 (2013).
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E. Rittweger, K. Y. Han, S. E. Irvine, C. Eggeling, and S. W. Hell, “STED microscopy reveals crystal colour centers with nanometric resolution,” Nat. Photonics 3, 144–147 (2009).
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S. Bounouar, M. Elouneg-Jamroz, M. den Hertog, C. Morchutt, E. Bellet-Amalric, R. André, C. Bougerol, Y. Genuist, J.-P. Poizat, S. Tatarenko, and K. Kheng, “Ultrafast room temperature single-photon source from nanowire-quantum dots,” Nano Lett. 12, 2977–2981 (2012).
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A. Karamlou, M. E. Trusheim, and D. Englund, “Metal-dielectric antennas for efficient photon collection from diamond color centers,” Opt. Express 26, 3341–3352 (2018).
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[Crossref]

I. Aharonovich, D. Englund, and M. Toth, “Solid-state single-photon emitters,” Nat. Photonics 10, 631–641 (2016).
[Crossref]

L. Li, E. H. Chen, J. Zheng, S. L. Mouradian, F. Dolde, T. Schröder, S. Karaveli, M. L. Markham, D. J. Twitchen, and D. Englund, “Efficient photon collection from a nitrogen vacancy center in a circular bullseye grating,” Nano Lett. 15, 1493–1497 (2015).
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Fairchild, B. A.

S. Castelletto, J. P. Harrison, L. Marseglia, A. C. Stanley-Clarke, B. C. Gibson, B. A. Fairchild, J. P. Hadden, Y.-L. D. Ho, M. P. Hiscocks, K. Ganesan, S. T. Huntington, F. Ladouceur, A. D. Greentree, S. Prawer, J. L. O’Brien, and J. G. Rarity, “Diamond-based structures to collect and guide light,” New J. Phys. 13, 025020 (2011).
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Fang, C.

G. M. Akselrod, C. Argyropoulos, T. B. Hoang, C. Ciracì, C. Fang, J. Huang, D. R. Smith, and M. H. Mikkelsen, “Probing the mechanisms of large Purcell enhancement in plasmonic nanoantennas,” Nat. Photonics 8, 835–840 (2014).
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Ferrera, M.

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Ford, M. J.

T. T. Tran, K. Bray, M. J. Ford, M. Toth, and I. Aharonovich, “Quantum emission from hexagonal boron nitride monolayers,” Nat. Nanotechnol. 11, 37–41 (2015).
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M. G. Blaber, M. D. Arnold, and M. J. Ford, “A review of the optical properties of alloys and intermetallics for plasmonics,” J. Phys. Condens. Matter 22, 143201 (2010).
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Gaebel, T.

F. A. Inam, M. D. W. Grogan, M. Rollings, T. Gaebel, J. M. Say, C. Bradac, T. A. Birks, W. J. Wadsworth, S. Castelletto, J. R. Rabeau, and M. J. Steel, “Emission and nonradiative decay of nanodiamond NV centers in a low refractive index environment,” ACS Nano 7, 3833–3843 (2013).
[Crossref]

F. A. Inam, T. Gaebel, C. Bradac, L. Stewart, M. J. Withford, J. M. Dawes, J. R. Rabeau, and M. J. Steel, “Modification of spontaneous emission from nano-diamond colour centers on a structured surface,” New J. Phys. 13, 073012 (2011).
[Crossref]

J. R. Rabeau, Y. L. Chin, S. Prawer, F. Jelezko, T. Gaebel, and J. Wrachtrup, “Fabrication of single nickel-nitrogen defects in diamond by chemical vapor deposition,” Appl. Phys. Lett. 86, 131926 (2005).
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Galfsky, T.

Ganesan, K.

S. Castelletto, J. P. Harrison, L. Marseglia, A. C. Stanley-Clarke, B. C. Gibson, B. A. Fairchild, J. P. Hadden, Y.-L. D. Ho, M. P. Hiscocks, K. Ganesan, S. T. Huntington, F. Ladouceur, A. D. Greentree, S. Prawer, J. L. O’Brien, and J. G. Rarity, “Diamond-based structures to collect and guide light,” New J. Phys. 13, 025020 (2011).
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S. Bounouar, M. Elouneg-Jamroz, M. den Hertog, C. Morchutt, E. Bellet-Amalric, R. André, C. Bougerol, Y. Genuist, J.-P. Poizat, S. Tatarenko, and K. Kheng, “Ultrafast room temperature single-photon source from nanowire-quantum dots,” Nano Lett. 12, 2977–2981 (2012).
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Gibson, B. C.

S. Castelletto, J. P. Harrison, L. Marseglia, A. C. Stanley-Clarke, B. C. Gibson, B. A. Fairchild, J. P. Hadden, Y.-L. D. Ho, M. P. Hiscocks, K. Ganesan, S. T. Huntington, F. Ladouceur, A. D. Greentree, S. Prawer, J. L. O’Brien, and J. G. Rarity, “Diamond-based structures to collect and guide light,” New J. Phys. 13, 025020 (2011).
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Figures (6)

Fig. 1.
Fig. 1. (a) Schematic image of the 5-layered Ag/Au-ZnS resonator. (b) The real and (c) the imaginary effective permittivity profile of the 5-layered Ag/Au-ZnS resonator structure as a function of wavelength.
Fig. 2.
Fig. 2. Schematic images of the 5-layered Ag-ZnS HMM resonator with (a) cylindrical Ag antenna and (b) hybrid metal–dielectric Ag-ZnS antenna on top. The dipole is considered to be oriented perpendicular to the Ag interface. The total performance of the above HMM resonator-antenna structures, (c) the “Relative” Purcell enhancement (${F_p}$), (d) the quantum efficiency (QE), (e) the collection efficiency (CE), and (f) the normalized collected photon counts (NCPC).
Fig. 3.
Fig. 3. Schematic images of the 5-layered Ag-ZnS cylindrical HMM resonator (a) with and (b) without cylindrical Ag antenna on top. The dipole is considered to be oriented perpendicular to the Ag/ZnS interface. The total performance of the above HMM resonator-antenna structures, (c) the “Relative” Purcell enhancement (${{\rm{F}}_p}$), (d) the quantum efficiency (QE), (e) the collection efficiency (CE), and (f) the normalized collected photon counts (NCPC).
Fig. 4.
Fig. 4. In-plane radiation pattern, ${|{\rm{E}}|^2}$ for dipole emission at 680 nm (a) on a glass substrate, inside a (b) HMM placed on a glass substrate with a ZnS DRA antenna, (c) HMM on glass substrate with a cylindrical Ag antenna, (d) HMM on glass with a hybrid Ag-ZnS antenna, (e) hybrid Ag-ZnS pillar resonator without antenna, and (f) hybrid Ag-ZnS pillar resonator with cylindrical Ag antenna.
Fig. 5.
Fig. 5. Far-field in-plane radiation pattern, ${|{{\rm{E}}_{\rm{far}}}|^2}$ for dipole emission at 680 nm (a) on a glass substrate, inside a (b) HMM placed on a glass substrate with a ZnS DRA antenna, (c) HMM on glass substrate with a cylindrical Ag antenna, (d) HMM on glass with hybrid Ag-ZnS antenna, (e) hybrid Ag-ZnS pillar resonator without antenna, and (f) hybrid Ag-ZnS pillar resonator with cylindrical Ag antenna.
Fig. 6.
Fig. 6. Simulated geometry of the 3D HMM structures, (a) 5-layered Ag-ZnS HMM structure with cylindrical hybrid metal (Ag) and dielectric (ZnS) antenna, and (b) 5-layered Ag-ZnS cylindrical HMM structure with cylindrical metallic Ag antenna.

Tables (1)

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Table 1. Comparison of the Best Performance of Some of the Recently Studied Resonator-Antenna Structures

Equations (1)

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Γ = π ω μ 2 k , σ | d ^ . E k , σ ( r ) | 2 δ ( ω ω k , σ ) .

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