Abstract

The electron–phonon coupling in self-assembled InGaAs quantum dots is relatively weak at low light intensities, which means that the zero-phonon line in emission is strong compared to the phonon sideband. However, the coupling to acoustic phonons can be dynamically enhanced in the presence of an intense optical pulse tuned within the phonon sideband. Recent experiments have shown that this dynamic vibronic coupling can enable population inversion to be achieved when pumping with a blueshifted laser and for rapid de-excitation of an inverted state with red detuning. In this paper we confirm the incoherent nature of the phonon-assisted pumping process and explore the temperature dependence of the mechanism. We also show that a combination of blueshifted and redshifted pulses can create and destroy an exciton within a timescale of 20  ps as determined by the pulse duration and ultimately limited by the phonon thermalization time.

© 2016 Optical Society of America

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References

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2016 (3)

F. Liu, L. M. P. Martins, A. J. Brash, A. M. Barth, J. H. Quilter, V. M. Axt, M. S. Skolnick, and A. M. Fox, “Ultrafast depopulation of a quantum dot by LA-phonon-assisted stimulated emission,” Phys. Rev. B 93, 161407(R) (2016).

J. Iles-Smith and A. Nazir, “Quantum correlations of light and matter through environmental transitions,” Optica 3, 207 (2016).
[Crossref]

F. Hargart, M. Müller, K. Roy-Choudhury, S. L. Portalupi, C. Schneider, S. Höfling, M. Kamp, S. Hughes, and P. Michler, “Cavity-enhanced simultaneous dressing of quantum dot exciton and biexciton states,” Phys. Rev. B 93, 115308 (2016).
[Crossref]

2015 (7)

D. Heinze, D. Breddermann, A. Zrenner, and S. Schumacher, “A quantum dot single-photon source with on-the-fly all-optical polarization control and timed emission,” Nat. Commun. 6, 8473 (2015).
[Crossref]

K. Müller, K. A. Fischer, A. Rundquist, C. Dory, K. G. Lagoudakis, T. Sarmiento, Y. A. Kelaita, V. Borish, and J. Vučković, “Ultrafast polariton-phonon dynamics of strongly coupled quantum dot-nanocavity systems,” Phys. Rev. X 5, 031006 (2015).

J. H. Quilter, A. J. Brash, F. Liu, M. Glässl, A. M. Barth, V. M. Axt, A. J. Ramsay, M. S. Skolnick, and A. M. Fox, “Phonon-assisted population inversion of a single InGaAs/GaAs quantum dot by pulsed laser excitation,” Phys. Rev. Lett. 114, 137401 (2015).
[Crossref]

S. Bounouar, M. Müller, A. M. Barth, M. Glässl, V. M. Axt, and P. Michler, “Phonon-assisted robust and deterministic two-photon biexciton preparation in a quantum dot,” Phys. Rev. B 91, 161302 (2015).
[Crossref]

A. J. Brash, L. M. P. P. Martins, F. Liu, J. H. Quilter, A. J. Ramsay, M. S. Skolnick, and A. M. Fox, “High-fidelity initialization of long-lived quantum dot hole spin qubits by reduced fine-structure splitting,” Phys. Rev. B 92, 121301 (2015).
[Crossref]

S. L. Portalupi, G. Hornecker, V. Giesz, T. Grange, A. Lemaître, J. Demory, I. Sagnes, N. D. Lanzillotti-Kimura, L. Lanco, A. Auffèves, and P. Senellart, “Bright phonon-tuned single-photon source,” Nano Lett. 15, 6290–6294 (2015).
[Crossref]

P. Lodahl, S. Mahmoodian, and S. Stobbe, “Interfacing single photons and single quantum dots with photonic nanostructures,” Rev. Mod. Phys. 87, 347–400 (2015).
[Crossref]

2014 (8)

R. Schirhagl, K. Chang, M. Loretz, and C. L. Degen, “Nitrogen-vacancy centers in diamond: nanoscale sensors for physics and biology,” Ann. Rev. Phys. Chem. 65, 83–105 (2014).
[Crossref]

P.-L. Ardelt, L. Hanschke, K. A. Fischer, K. Müller, A. Kleinkauf, M. Koller, A. Bechtold, T. Simmet, J. Wierzbowski, H. Riedl, G. Abstreiter, and J. J. Finley, “Dissipative preparation of the exciton and biexciton in self-assembled quantum dots on picosecond time scales,” Phys. Rev. B 90, 241404(R) (2014).
[Crossref]

K. H. Madsen, S. Ates, J. Liu, A. Javadi, S. M. Albrecht, I. Yeo, S. Stobbe, and P. Lodahl, “Efficient out-coupling of high-purity single photons from a coherent quantum dot in a photonic-crystal cavity,” Phys. Rev. B 90, 155303 (2014).
[Crossref]

J. Hansom, C. H. H. Schulte, C. Matthiesen, M. J. Stanley, and M. Atatüre, “Frequency stabilization of the zero-phonon line of a quantum dot via phonon-assisted active feedback,” Appl. Phys. Lett. 105, 172107 (2014).
[Crossref]

Y. J. Wei, Y. M. He, M. C. Chen, Y. N. Hu, Y. He, D. Wu, C. Schneider, M. Kamp, S. Höfling, C. Y. Lu, and J.-W. Pan, “Deterministic and robust generation of single photons from a single quantum dot with 99.5% indistinguishably using adiabatic rapid passage,” Nano Lett. 14, 6515–6519 (2014).
[Crossref]

R. Mathew, E. Dilcher, A. Gamouras, A. Ramachandran, H. Y. Shi Yang, S. Freisem, D. Deppe, and K. C. Hall, “Subpicosecond adiabatic rapid passage on a single semiconductor quantum dot: phonon-mediated dephasing in the strong-driving regime,” Phys. Rev. B 90, 035316 (2014).
[Crossref]

Y.-J. Wei, Y. He, Y.-M. He, C.-Y. Lu, J.-W. Pan, C. Schneider, M. Kamp, S. Höfling, D. P. S. McCutcheon, and A. Nazir, “Temperature-dependent Mollow triplet spectra from a single quantum dot: Rabi frequency renormalization and sideband linewidth insensitivity,” Phys. Rev. Lett. 113, 097401 (2014).
[Crossref]

E. Cancellieri, A. Hayat, A. M. Steinberg, E. Giacobino, and A. Bramati, “Ultrafast Stark-induced polaritonic switches,” Phys. Rev. Lett. 112, 053601 (2014).
[Crossref]

2013 (4)

S. Hughes and H. J. Carmichael, “Phonon-mediated population inversion in a semiconductor quantum-dot cavity system,” New J. Phys. 15, 053039 (2013).
[Crossref]

D. P. S. McCutcheon and A. Nazir, “Model of the optical emission of a driven semiconductor quantum dot: phonon-enhanced coherent scattering and off-resonant sideband narrowing,” Phys. Rev. Lett. 110, 217401 (2013).
[Crossref]

L. Monniello, C. Tonin, R. Hostein, A. Lemaitre, A. Martinez, V. Voliotis, and R. Grousson, “Excitation-induced dephasing in a resonantly driven InAs/GaAs quantum dot,” Phys. Rev. Lett. 111, 026403 (2013).
[Crossref]

M. Glässl, A. M. Barth, and V. M. Axt, “Proposed robust and high-fidelity preparation of excitons and biexcitons in semiconductor quantum dots making active use of phonons,” Phys. Rev. Lett. 110, 147401 (2013).
[Crossref]

2012 (3)

S. Weiler, A. Ulhaq, S. M. Ulrich, D. Richter, M. Jetter, P. Michler, C. Roy, and S. Hughes, “Phonon-assisted incoherent excitation of a quantum dot and its emission properties,” Phys. Rev. B 86, 241304(R) (2012).
[Crossref]

T. M. Godden, J. H. Quilter, A. J. Ramsay, Y. Wu, P. Brereton, S. J. Boyle, I. J. Luxmoore, J. Puebla-Nunez, A. M. Fox, and M. S. Skolnick, “Coherent optical control of the spin of a single hole in an InAs/GaAs quantum dot,” Phys. Rev. Lett. 108, 017402 (2012).
[Crossref]

T. Volz, A. Reinhard, M. Winger, A. Badolato, K. J. Hennessy, E. L. Hu, and A. Imamoglu, “Ultrafast all-optical switching by single photons,” Nat. Photonics 6, 607–611 (2012).
[Crossref]

2011 (1)

A. J. Ramsay, T. M. Godden, S. J. Boyle, E. M. Gauger, A. Nazir, B. W. Lovett, A. V. Gopal, A. M. Fox, and M. S. Skolnick, “Effect of detuning on the phonon induced dephasing of optically driven InGaAs/GaAs quantum dots,” J. Appl. Phys. 109, 102415 (2011).
[Crossref]

2010 (5)

A. J. Ramsay, A. V. Gopal, E. M. Gauger, A. Nazir, B. W. Lovett, A. M. Fox, and M. S. Skolnick, “Damping of exciton Rabi rotations by acoustic phonons in optically excited InGaAs/GaAs quantum dots,” Phys. Rev. Lett. 104, 017402 (2010).
[Crossref]

D. P. S. McCutcheon and A. Nazir, “Quantum dot Rabi rotations beyond the weak exciton-phonon coupling regime,” New J. Phys. 12, 113042 (2010).
[Crossref]

A. J. Ramsay, T. M. Godden, S. J. Boyle, E. M. Gauger, A. Nazir, B. W. Lovett, A. M. Fox, and M. S. Skolnick, “Phonon-induced Rabi-frequency renormalization of optically driven single InGaAs/GaAs quantum dots,” Phys. Rev. Lett. 105, 177402 (2010).
[Crossref]

J. Klein and J. D. Kafka, “The Ti:sapphire laser: the flexible research tool,” Nat. Photonics 4, 289 (2010).
[Crossref]

M. Nomura, N. Kumagai, S. Iwamoto, Y. Ota, and Y. Arakawa, “Laser oscillation in a strongly coupled single-quantum-dot-nanocavity system,” Nat. Phys. 6, 279–283 (2010).
[Crossref]

2009 (2)

S. Ates, S. M. Ulrich, A. Ulhaq, S. Reitzenstein, A. Löffler, S. Höfling, A. Forchel, and P. Michler, “Non-resonant dot-cavity coupling and its potential for resonant single-quantum-dot-spectroscopy,” Nat. Photonics 3, 724–728 (2009).
[Crossref]

S. J. Boyle, A. J. Ramsay, A. M. Fox, M. S. Skolnick, A. P. Heberle, and M. Hopkinson, “Beating of exciton dressed states in a single semiconductor InGaAs/GaAs quantum dot,” Phys. Rev. Lett. 102, 207401 (2009).
[Crossref]

2008 (2)

S. J. Boyle, A. J. Ramsay, F. Bello, H. Y. Liu, M. Hopkinson, A. M. Fox, and M. S. Skolnick, “Two-qubit conditional quantum-logic operation in a single self-assembled quantum dot,” Phys. Rev. B 78, 075301 (2008).
[Crossref]

P. A. Dalgarno, J. M. Smith, J. McFarlane, B. D. Gerardot, K. Karrai, A. Badolato, P. M. Petroff, and R. J. Warburton, “Coulomb interactions in single charged self-assembled quantum dots: radiative lifetime and recombination energy,” Phys. Rev. B 77, 245311 (2008).
[Crossref]

2007 (1)

R. S. Kolodka, A. J. Ramsay, J. Skiba-Szymanska, P. W. Fry, H. Y. Liu, A. M. Fox, and M. S. Skolnick, “Inversion recovery of single quantum-dot exciton based qubit,” Phys. Rev. B 75, 193306(R) (2007).
[Crossref]

2005 (2)

S. Stufler, P. Ester, A. Zrenner, and M. Bichler, “Exciton Rabi oscillation in a single quantum dot,” Phys. Rev. B 72, 121301(R) (2005).
[Crossref]

P. Borri, W. Langbein, U. Woggon, V. Stavarache, D. Reuter, and A. Wieck, “Exciton dephasing via phonon interactions in InAs quantum dots: dependence on quantum confinement,” Phys. Rev. B 71, 115328 (2005).
[Crossref]

2003 (1)

I. Favero, G. Cassabois, R. Ferreira, D. Darson, C. Voisin, J. Tignon, C. Delalande, G. Bastard, and Ph. Roussignol, “Acoustic phonon sidebands in the emission line of single InAs/GaAs quantum dots,” Phys. Rev. B 68, 233301 (2003).
[Crossref]

2002 (2)

A. Zrenner, E. Beham, S. Stuer, F. Findeis, M. Bichler, and G. Abstreiter, “Coherent properties of a two-level system based on a quantum-dot photodiode,” Nature 418, 612–614 (2002).
[Crossref]

B. Krummheuer, V. M. Axt, and T. Kuhn, “Theory of pure dephasing and the resulting absorption line shape in semiconductor quantum dots,” Phys. Rev. B 65, 195313 (2002).
[Crossref]

2001 (2)

H. Kamada, H. Gotoh, J. Temmyo, T. Takagahara, and H. Ando, “Exciton Rabi oscillation in a single quantum dot,” Phys. Rev. Lett. 87, 246401 (2001).
[Crossref]

P. Borri, W. Langbein, S. Schneider, U. Woggon, R. L. Sellin, D. Ouyang, and D. Bimberg, “Ultralong dephasing time in InGaAs quantum dots,” Phys. Rev. Lett. 87, 157401 (2001).
[Crossref]

2000 (1)

P. G. Eliseev, H. Li, A. Stintz, G. T. Liu, T. C. Newell, K. J. Malloy, and L. F. Lester, “Transition dipole moment of InAs/InGaAs quantum dots from experiments on ultralow-threshold laser diodes,” Appl. Phys. Lett. 77, 262–264 (2000).
[Crossref]

1995 (1)

A. P. Heberle and J. J. Baumberg, “Ultrafast coherent control and destruction of excitons in quantum wells,” Phys. Rev. Lett. 75, 2598–2601 (1995).
[Crossref]

1981 (1)

G. Davies, “The Jahn-Teller effect and vibronic coupling at deep levels in diamond,” Rep. Prog. Phys. 44, 787–830 (1981).
[Crossref]

1976 (1)

G. Davies and M. F. Hamer, “Optical studies of the 1.945  eV vibronic band in diamond,” Proc. R. Soc. Lond. A 348, 285–298 (1976).
[Crossref]

Abstreiter, G.

P.-L. Ardelt, L. Hanschke, K. A. Fischer, K. Müller, A. Kleinkauf, M. Koller, A. Bechtold, T. Simmet, J. Wierzbowski, H. Riedl, G. Abstreiter, and J. J. Finley, “Dissipative preparation of the exciton and biexciton in self-assembled quantum dots on picosecond time scales,” Phys. Rev. B 90, 241404(R) (2014).
[Crossref]

A. Zrenner, E. Beham, S. Stuer, F. Findeis, M. Bichler, and G. Abstreiter, “Coherent properties of a two-level system based on a quantum-dot photodiode,” Nature 418, 612–614 (2002).
[Crossref]

Albrecht, S. M.

K. H. Madsen, S. Ates, J. Liu, A. Javadi, S. M. Albrecht, I. Yeo, S. Stobbe, and P. Lodahl, “Efficient out-coupling of high-purity single photons from a coherent quantum dot in a photonic-crystal cavity,” Phys. Rev. B 90, 155303 (2014).
[Crossref]

Ando, H.

H. Kamada, H. Gotoh, J. Temmyo, T. Takagahara, and H. Ando, “Exciton Rabi oscillation in a single quantum dot,” Phys. Rev. Lett. 87, 246401 (2001).
[Crossref]

Arakawa, Y.

M. Nomura, N. Kumagai, S. Iwamoto, Y. Ota, and Y. Arakawa, “Laser oscillation in a strongly coupled single-quantum-dot-nanocavity system,” Nat. Phys. 6, 279–283 (2010).
[Crossref]

Ardelt, P.-L.

P.-L. Ardelt, L. Hanschke, K. A. Fischer, K. Müller, A. Kleinkauf, M. Koller, A. Bechtold, T. Simmet, J. Wierzbowski, H. Riedl, G. Abstreiter, and J. J. Finley, “Dissipative preparation of the exciton and biexciton in self-assembled quantum dots on picosecond time scales,” Phys. Rev. B 90, 241404(R) (2014).
[Crossref]

Atatüre, M.

J. Hansom, C. H. H. Schulte, C. Matthiesen, M. J. Stanley, and M. Atatüre, “Frequency stabilization of the zero-phonon line of a quantum dot via phonon-assisted active feedback,” Appl. Phys. Lett. 105, 172107 (2014).
[Crossref]

Ates, S.

K. H. Madsen, S. Ates, J. Liu, A. Javadi, S. M. Albrecht, I. Yeo, S. Stobbe, and P. Lodahl, “Efficient out-coupling of high-purity single photons from a coherent quantum dot in a photonic-crystal cavity,” Phys. Rev. B 90, 155303 (2014).
[Crossref]

S. Ates, S. M. Ulrich, A. Ulhaq, S. Reitzenstein, A. Löffler, S. Höfling, A. Forchel, and P. Michler, “Non-resonant dot-cavity coupling and its potential for resonant single-quantum-dot-spectroscopy,” Nat. Photonics 3, 724–728 (2009).
[Crossref]

Auffèves, A.

S. L. Portalupi, G. Hornecker, V. Giesz, T. Grange, A. Lemaître, J. Demory, I. Sagnes, N. D. Lanzillotti-Kimura, L. Lanco, A. Auffèves, and P. Senellart, “Bright phonon-tuned single-photon source,” Nano Lett. 15, 6290–6294 (2015).
[Crossref]

Axt, V. M.

F. Liu, L. M. P. Martins, A. J. Brash, A. M. Barth, J. H. Quilter, V. M. Axt, M. S. Skolnick, and A. M. Fox, “Ultrafast depopulation of a quantum dot by LA-phonon-assisted stimulated emission,” Phys. Rev. B 93, 161407(R) (2016).

S. Bounouar, M. Müller, A. M. Barth, M. Glässl, V. M. Axt, and P. Michler, “Phonon-assisted robust and deterministic two-photon biexciton preparation in a quantum dot,” Phys. Rev. B 91, 161302 (2015).
[Crossref]

J. H. Quilter, A. J. Brash, F. Liu, M. Glässl, A. M. Barth, V. M. Axt, A. J. Ramsay, M. S. Skolnick, and A. M. Fox, “Phonon-assisted population inversion of a single InGaAs/GaAs quantum dot by pulsed laser excitation,” Phys. Rev. Lett. 114, 137401 (2015).
[Crossref]

M. Glässl, A. M. Barth, and V. M. Axt, “Proposed robust and high-fidelity preparation of excitons and biexcitons in semiconductor quantum dots making active use of phonons,” Phys. Rev. Lett. 110, 147401 (2013).
[Crossref]

B. Krummheuer, V. M. Axt, and T. Kuhn, “Theory of pure dephasing and the resulting absorption line shape in semiconductor quantum dots,” Phys. Rev. B 65, 195313 (2002).
[Crossref]

A. M. Barth, S. Lüker, A. Vagov, D. E. Reiter, T. Kuhn, and V. M. Axt, “Fast and selective phonon-assisted state preparation of a quantum dot by adiabatic undressing,” Phys. Rev. B, arXiv:1601.07886 (to be published).

Badolato, A.

T. Volz, A. Reinhard, M. Winger, A. Badolato, K. J. Hennessy, E. L. Hu, and A. Imamoglu, “Ultrafast all-optical switching by single photons,” Nat. Photonics 6, 607–611 (2012).
[Crossref]

P. A. Dalgarno, J. M. Smith, J. McFarlane, B. D. Gerardot, K. Karrai, A. Badolato, P. M. Petroff, and R. J. Warburton, “Coulomb interactions in single charged self-assembled quantum dots: radiative lifetime and recombination energy,” Phys. Rev. B 77, 245311 (2008).
[Crossref]

Barth, A. M.

F. Liu, L. M. P. Martins, A. J. Brash, A. M. Barth, J. H. Quilter, V. M. Axt, M. S. Skolnick, and A. M. Fox, “Ultrafast depopulation of a quantum dot by LA-phonon-assisted stimulated emission,” Phys. Rev. B 93, 161407(R) (2016).

J. H. Quilter, A. J. Brash, F. Liu, M. Glässl, A. M. Barth, V. M. Axt, A. J. Ramsay, M. S. Skolnick, and A. M. Fox, “Phonon-assisted population inversion of a single InGaAs/GaAs quantum dot by pulsed laser excitation,” Phys. Rev. Lett. 114, 137401 (2015).
[Crossref]

S. Bounouar, M. Müller, A. M. Barth, M. Glässl, V. M. Axt, and P. Michler, “Phonon-assisted robust and deterministic two-photon biexciton preparation in a quantum dot,” Phys. Rev. B 91, 161302 (2015).
[Crossref]

M. Glässl, A. M. Barth, and V. M. Axt, “Proposed robust and high-fidelity preparation of excitons and biexcitons in semiconductor quantum dots making active use of phonons,” Phys. Rev. Lett. 110, 147401 (2013).
[Crossref]

A. M. Barth, S. Lüker, A. Vagov, D. E. Reiter, T. Kuhn, and V. M. Axt, “Fast and selective phonon-assisted state preparation of a quantum dot by adiabatic undressing,” Phys. Rev. B, arXiv:1601.07886 (to be published).

Bastard, G.

I. Favero, G. Cassabois, R. Ferreira, D. Darson, C. Voisin, J. Tignon, C. Delalande, G. Bastard, and Ph. Roussignol, “Acoustic phonon sidebands in the emission line of single InAs/GaAs quantum dots,” Phys. Rev. B 68, 233301 (2003).
[Crossref]

Baumberg, J. J.

A. P. Heberle and J. J. Baumberg, “Ultrafast coherent control and destruction of excitons in quantum wells,” Phys. Rev. Lett. 75, 2598–2601 (1995).
[Crossref]

Bechtold, A.

P.-L. Ardelt, L. Hanschke, K. A. Fischer, K. Müller, A. Kleinkauf, M. Koller, A. Bechtold, T. Simmet, J. Wierzbowski, H. Riedl, G. Abstreiter, and J. J. Finley, “Dissipative preparation of the exciton and biexciton in self-assembled quantum dots on picosecond time scales,” Phys. Rev. B 90, 241404(R) (2014).
[Crossref]

Beham, E.

A. Zrenner, E. Beham, S. Stuer, F. Findeis, M. Bichler, and G. Abstreiter, “Coherent properties of a two-level system based on a quantum-dot photodiode,” Nature 418, 612–614 (2002).
[Crossref]

Bello, F.

S. J. Boyle, A. J. Ramsay, F. Bello, H. Y. Liu, M. Hopkinson, A. M. Fox, and M. S. Skolnick, “Two-qubit conditional quantum-logic operation in a single self-assembled quantum dot,” Phys. Rev. B 78, 075301 (2008).
[Crossref]

Bichler, M.

S. Stufler, P. Ester, A. Zrenner, and M. Bichler, “Exciton Rabi oscillation in a single quantum dot,” Phys. Rev. B 72, 121301(R) (2005).
[Crossref]

A. Zrenner, E. Beham, S. Stuer, F. Findeis, M. Bichler, and G. Abstreiter, “Coherent properties of a two-level system based on a quantum-dot photodiode,” Nature 418, 612–614 (2002).
[Crossref]

Bimberg, D.

P. Borri, W. Langbein, S. Schneider, U. Woggon, R. L. Sellin, D. Ouyang, and D. Bimberg, “Ultralong dephasing time in InGaAs quantum dots,” Phys. Rev. Lett. 87, 157401 (2001).
[Crossref]

Borish, V.

K. Müller, K. A. Fischer, A. Rundquist, C. Dory, K. G. Lagoudakis, T. Sarmiento, Y. A. Kelaita, V. Borish, and J. Vučković, “Ultrafast polariton-phonon dynamics of strongly coupled quantum dot-nanocavity systems,” Phys. Rev. X 5, 031006 (2015).

Borri, P.

P. Borri, W. Langbein, U. Woggon, V. Stavarache, D. Reuter, and A. Wieck, “Exciton dephasing via phonon interactions in InAs quantum dots: dependence on quantum confinement,” Phys. Rev. B 71, 115328 (2005).
[Crossref]

P. Borri, W. Langbein, S. Schneider, U. Woggon, R. L. Sellin, D. Ouyang, and D. Bimberg, “Ultralong dephasing time in InGaAs quantum dots,” Phys. Rev. Lett. 87, 157401 (2001).
[Crossref]

Bounouar, S.

S. Bounouar, M. Müller, A. M. Barth, M. Glässl, V. M. Axt, and P. Michler, “Phonon-assisted robust and deterministic two-photon biexciton preparation in a quantum dot,” Phys. Rev. B 91, 161302 (2015).
[Crossref]

Boyle, S. J.

T. M. Godden, J. H. Quilter, A. J. Ramsay, Y. Wu, P. Brereton, S. J. Boyle, I. J. Luxmoore, J. Puebla-Nunez, A. M. Fox, and M. S. Skolnick, “Coherent optical control of the spin of a single hole in an InAs/GaAs quantum dot,” Phys. Rev. Lett. 108, 017402 (2012).
[Crossref]

A. J. Ramsay, T. M. Godden, S. J. Boyle, E. M. Gauger, A. Nazir, B. W. Lovett, A. V. Gopal, A. M. Fox, and M. S. Skolnick, “Effect of detuning on the phonon induced dephasing of optically driven InGaAs/GaAs quantum dots,” J. Appl. Phys. 109, 102415 (2011).
[Crossref]

A. J. Ramsay, T. M. Godden, S. J. Boyle, E. M. Gauger, A. Nazir, B. W. Lovett, A. M. Fox, and M. S. Skolnick, “Phonon-induced Rabi-frequency renormalization of optically driven single InGaAs/GaAs quantum dots,” Phys. Rev. Lett. 105, 177402 (2010).
[Crossref]

S. J. Boyle, A. J. Ramsay, A. M. Fox, M. S. Skolnick, A. P. Heberle, and M. Hopkinson, “Beating of exciton dressed states in a single semiconductor InGaAs/GaAs quantum dot,” Phys. Rev. Lett. 102, 207401 (2009).
[Crossref]

S. J. Boyle, A. J. Ramsay, F. Bello, H. Y. Liu, M. Hopkinson, A. M. Fox, and M. S. Skolnick, “Two-qubit conditional quantum-logic operation in a single self-assembled quantum dot,” Phys. Rev. B 78, 075301 (2008).
[Crossref]

Bramati, A.

E. Cancellieri, A. Hayat, A. M. Steinberg, E. Giacobino, and A. Bramati, “Ultrafast Stark-induced polaritonic switches,” Phys. Rev. Lett. 112, 053601 (2014).
[Crossref]

Brash, A. J.

F. Liu, L. M. P. Martins, A. J. Brash, A. M. Barth, J. H. Quilter, V. M. Axt, M. S. Skolnick, and A. M. Fox, “Ultrafast depopulation of a quantum dot by LA-phonon-assisted stimulated emission,” Phys. Rev. B 93, 161407(R) (2016).

A. J. Brash, L. M. P. P. Martins, F. Liu, J. H. Quilter, A. J. Ramsay, M. S. Skolnick, and A. M. Fox, “High-fidelity initialization of long-lived quantum dot hole spin qubits by reduced fine-structure splitting,” Phys. Rev. B 92, 121301 (2015).
[Crossref]

J. H. Quilter, A. J. Brash, F. Liu, M. Glässl, A. M. Barth, V. M. Axt, A. J. Ramsay, M. S. Skolnick, and A. M. Fox, “Phonon-assisted population inversion of a single InGaAs/GaAs quantum dot by pulsed laser excitation,” Phys. Rev. Lett. 114, 137401 (2015).
[Crossref]

Breddermann, D.

D. Heinze, D. Breddermann, A. Zrenner, and S. Schumacher, “A quantum dot single-photon source with on-the-fly all-optical polarization control and timed emission,” Nat. Commun. 6, 8473 (2015).
[Crossref]

Brereton, P.

T. M. Godden, J. H. Quilter, A. J. Ramsay, Y. Wu, P. Brereton, S. J. Boyle, I. J. Luxmoore, J. Puebla-Nunez, A. M. Fox, and M. S. Skolnick, “Coherent optical control of the spin of a single hole in an InAs/GaAs quantum dot,” Phys. Rev. Lett. 108, 017402 (2012).
[Crossref]

Cancellieri, E.

E. Cancellieri, A. Hayat, A. M. Steinberg, E. Giacobino, and A. Bramati, “Ultrafast Stark-induced polaritonic switches,” Phys. Rev. Lett. 112, 053601 (2014).
[Crossref]

Carmichael, H. J.

S. Hughes and H. J. Carmichael, “Phonon-mediated population inversion in a semiconductor quantum-dot cavity system,” New J. Phys. 15, 053039 (2013).
[Crossref]

Cassabois, G.

I. Favero, G. Cassabois, R. Ferreira, D. Darson, C. Voisin, J. Tignon, C. Delalande, G. Bastard, and Ph. Roussignol, “Acoustic phonon sidebands in the emission line of single InAs/GaAs quantum dots,” Phys. Rev. B 68, 233301 (2003).
[Crossref]

Chang, K.

R. Schirhagl, K. Chang, M. Loretz, and C. L. Degen, “Nitrogen-vacancy centers in diamond: nanoscale sensors for physics and biology,” Ann. Rev. Phys. Chem. 65, 83–105 (2014).
[Crossref]

Chen, M. C.

Y. J. Wei, Y. M. He, M. C. Chen, Y. N. Hu, Y. He, D. Wu, C. Schneider, M. Kamp, S. Höfling, C. Y. Lu, and J.-W. Pan, “Deterministic and robust generation of single photons from a single quantum dot with 99.5% indistinguishably using adiabatic rapid passage,” Nano Lett. 14, 6515–6519 (2014).
[Crossref]

Dalgarno, P. A.

P. A. Dalgarno, J. M. Smith, J. McFarlane, B. D. Gerardot, K. Karrai, A. Badolato, P. M. Petroff, and R. J. Warburton, “Coulomb interactions in single charged self-assembled quantum dots: radiative lifetime and recombination energy,” Phys. Rev. B 77, 245311 (2008).
[Crossref]

Darson, D.

I. Favero, G. Cassabois, R. Ferreira, D. Darson, C. Voisin, J. Tignon, C. Delalande, G. Bastard, and Ph. Roussignol, “Acoustic phonon sidebands in the emission line of single InAs/GaAs quantum dots,” Phys. Rev. B 68, 233301 (2003).
[Crossref]

Davies, G.

G. Davies, “The Jahn-Teller effect and vibronic coupling at deep levels in diamond,” Rep. Prog. Phys. 44, 787–830 (1981).
[Crossref]

G. Davies and M. F. Hamer, “Optical studies of the 1.945  eV vibronic band in diamond,” Proc. R. Soc. Lond. A 348, 285–298 (1976).
[Crossref]

De Silvestri, S.

O. Svelto, S. De Silvestri, and G. Denardo, Ultrafast Processes in Spectroscopy (Springer, 1996).

Degen, C. L.

R. Schirhagl, K. Chang, M. Loretz, and C. L. Degen, “Nitrogen-vacancy centers in diamond: nanoscale sensors for physics and biology,” Ann. Rev. Phys. Chem. 65, 83–105 (2014).
[Crossref]

Delalande, C.

I. Favero, G. Cassabois, R. Ferreira, D. Darson, C. Voisin, J. Tignon, C. Delalande, G. Bastard, and Ph. Roussignol, “Acoustic phonon sidebands in the emission line of single InAs/GaAs quantum dots,” Phys. Rev. B 68, 233301 (2003).
[Crossref]

Demory, J.

S. L. Portalupi, G. Hornecker, V. Giesz, T. Grange, A. Lemaître, J. Demory, I. Sagnes, N. D. Lanzillotti-Kimura, L. Lanco, A. Auffèves, and P. Senellart, “Bright phonon-tuned single-photon source,” Nano Lett. 15, 6290–6294 (2015).
[Crossref]

Denardo, G.

O. Svelto, S. De Silvestri, and G. Denardo, Ultrafast Processes in Spectroscopy (Springer, 1996).

Deppe, D.

R. Mathew, E. Dilcher, A. Gamouras, A. Ramachandran, H. Y. Shi Yang, S. Freisem, D. Deppe, and K. C. Hall, “Subpicosecond adiabatic rapid passage on a single semiconductor quantum dot: phonon-mediated dephasing in the strong-driving regime,” Phys. Rev. B 90, 035316 (2014).
[Crossref]

Dilcher, E.

R. Mathew, E. Dilcher, A. Gamouras, A. Ramachandran, H. Y. Shi Yang, S. Freisem, D. Deppe, and K. C. Hall, “Subpicosecond adiabatic rapid passage on a single semiconductor quantum dot: phonon-mediated dephasing in the strong-driving regime,” Phys. Rev. B 90, 035316 (2014).
[Crossref]

Dory, C.

K. Müller, K. A. Fischer, A. Rundquist, C. Dory, K. G. Lagoudakis, T. Sarmiento, Y. A. Kelaita, V. Borish, and J. Vučković, “Ultrafast polariton-phonon dynamics of strongly coupled quantum dot-nanocavity systems,” Phys. Rev. X 5, 031006 (2015).

Eliseev, P. G.

P. G. Eliseev, H. Li, A. Stintz, G. T. Liu, T. C. Newell, K. J. Malloy, and L. F. Lester, “Transition dipole moment of InAs/InGaAs quantum dots from experiments on ultralow-threshold laser diodes,” Appl. Phys. Lett. 77, 262–264 (2000).
[Crossref]

Ester, P.

S. Stufler, P. Ester, A. Zrenner, and M. Bichler, “Exciton Rabi oscillation in a single quantum dot,” Phys. Rev. B 72, 121301(R) (2005).
[Crossref]

Favero, I.

I. Favero, G. Cassabois, R. Ferreira, D. Darson, C. Voisin, J. Tignon, C. Delalande, G. Bastard, and Ph. Roussignol, “Acoustic phonon sidebands in the emission line of single InAs/GaAs quantum dots,” Phys. Rev. B 68, 233301 (2003).
[Crossref]

Ferreira, R.

I. Favero, G. Cassabois, R. Ferreira, D. Darson, C. Voisin, J. Tignon, C. Delalande, G. Bastard, and Ph. Roussignol, “Acoustic phonon sidebands in the emission line of single InAs/GaAs quantum dots,” Phys. Rev. B 68, 233301 (2003).
[Crossref]

Findeis, F.

A. Zrenner, E. Beham, S. Stuer, F. Findeis, M. Bichler, and G. Abstreiter, “Coherent properties of a two-level system based on a quantum-dot photodiode,” Nature 418, 612–614 (2002).
[Crossref]

Finley, J. J.

P.-L. Ardelt, L. Hanschke, K. A. Fischer, K. Müller, A. Kleinkauf, M. Koller, A. Bechtold, T. Simmet, J. Wierzbowski, H. Riedl, G. Abstreiter, and J. J. Finley, “Dissipative preparation of the exciton and biexciton in self-assembled quantum dots on picosecond time scales,” Phys. Rev. B 90, 241404(R) (2014).
[Crossref]

Fischer, K. A.

K. Müller, K. A. Fischer, A. Rundquist, C. Dory, K. G. Lagoudakis, T. Sarmiento, Y. A. Kelaita, V. Borish, and J. Vučković, “Ultrafast polariton-phonon dynamics of strongly coupled quantum dot-nanocavity systems,” Phys. Rev. X 5, 031006 (2015).

P.-L. Ardelt, L. Hanschke, K. A. Fischer, K. Müller, A. Kleinkauf, M. Koller, A. Bechtold, T. Simmet, J. Wierzbowski, H. Riedl, G. Abstreiter, and J. J. Finley, “Dissipative preparation of the exciton and biexciton in self-assembled quantum dots on picosecond time scales,” Phys. Rev. B 90, 241404(R) (2014).
[Crossref]

Forchel, A.

S. Ates, S. M. Ulrich, A. Ulhaq, S. Reitzenstein, A. Löffler, S. Höfling, A. Forchel, and P. Michler, “Non-resonant dot-cavity coupling and its potential for resonant single-quantum-dot-spectroscopy,” Nat. Photonics 3, 724–728 (2009).
[Crossref]

Fox, A. M.

F. Liu, L. M. P. Martins, A. J. Brash, A. M. Barth, J. H. Quilter, V. M. Axt, M. S. Skolnick, and A. M. Fox, “Ultrafast depopulation of a quantum dot by LA-phonon-assisted stimulated emission,” Phys. Rev. B 93, 161407(R) (2016).

J. H. Quilter, A. J. Brash, F. Liu, M. Glässl, A. M. Barth, V. M. Axt, A. J. Ramsay, M. S. Skolnick, and A. M. Fox, “Phonon-assisted population inversion of a single InGaAs/GaAs quantum dot by pulsed laser excitation,” Phys. Rev. Lett. 114, 137401 (2015).
[Crossref]

A. J. Brash, L. M. P. P. Martins, F. Liu, J. H. Quilter, A. J. Ramsay, M. S. Skolnick, and A. M. Fox, “High-fidelity initialization of long-lived quantum dot hole spin qubits by reduced fine-structure splitting,” Phys. Rev. B 92, 121301 (2015).
[Crossref]

T. M. Godden, J. H. Quilter, A. J. Ramsay, Y. Wu, P. Brereton, S. J. Boyle, I. J. Luxmoore, J. Puebla-Nunez, A. M. Fox, and M. S. Skolnick, “Coherent optical control of the spin of a single hole in an InAs/GaAs quantum dot,” Phys. Rev. Lett. 108, 017402 (2012).
[Crossref]

A. J. Ramsay, T. M. Godden, S. J. Boyle, E. M. Gauger, A. Nazir, B. W. Lovett, A. V. Gopal, A. M. Fox, and M. S. Skolnick, “Effect of detuning on the phonon induced dephasing of optically driven InGaAs/GaAs quantum dots,” J. Appl. Phys. 109, 102415 (2011).
[Crossref]

A. J. Ramsay, A. V. Gopal, E. M. Gauger, A. Nazir, B. W. Lovett, A. M. Fox, and M. S. Skolnick, “Damping of exciton Rabi rotations by acoustic phonons in optically excited InGaAs/GaAs quantum dots,” Phys. Rev. Lett. 104, 017402 (2010).
[Crossref]

A. J. Ramsay, T. M. Godden, S. J. Boyle, E. M. Gauger, A. Nazir, B. W. Lovett, A. M. Fox, and M. S. Skolnick, “Phonon-induced Rabi-frequency renormalization of optically driven single InGaAs/GaAs quantum dots,” Phys. Rev. Lett. 105, 177402 (2010).
[Crossref]

S. J. Boyle, A. J. Ramsay, A. M. Fox, M. S. Skolnick, A. P. Heberle, and M. Hopkinson, “Beating of exciton dressed states in a single semiconductor InGaAs/GaAs quantum dot,” Phys. Rev. Lett. 102, 207401 (2009).
[Crossref]

S. J. Boyle, A. J. Ramsay, F. Bello, H. Y. Liu, M. Hopkinson, A. M. Fox, and M. S. Skolnick, “Two-qubit conditional quantum-logic operation in a single self-assembled quantum dot,” Phys. Rev. B 78, 075301 (2008).
[Crossref]

R. S. Kolodka, A. J. Ramsay, J. Skiba-Szymanska, P. W. Fry, H. Y. Liu, A. M. Fox, and M. S. Skolnick, “Inversion recovery of single quantum-dot exciton based qubit,” Phys. Rev. B 75, 193306(R) (2007).
[Crossref]

Fox, M.

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S. Ates, S. M. Ulrich, A. Ulhaq, S. Reitzenstein, A. Löffler, S. Höfling, A. Forchel, and P. Michler, “Non-resonant dot-cavity coupling and its potential for resonant single-quantum-dot-spectroscopy,” Nat. Photonics 3, 724–728 (2009).
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R. Schirhagl, K. Chang, M. Loretz, and C. L. Degen, “Nitrogen-vacancy centers in diamond: nanoscale sensors for physics and biology,” Ann. Rev. Phys. Chem. 65, 83–105 (2014).
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A. J. Ramsay, T. M. Godden, S. J. Boyle, E. M. Gauger, A. Nazir, B. W. Lovett, A. V. Gopal, A. M. Fox, and M. S. Skolnick, “Effect of detuning on the phonon induced dephasing of optically driven InGaAs/GaAs quantum dots,” J. Appl. Phys. 109, 102415 (2011).
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A. J. Ramsay, A. V. Gopal, E. M. Gauger, A. Nazir, B. W. Lovett, A. M. Fox, and M. S. Skolnick, “Damping of exciton Rabi rotations by acoustic phonons in optically excited InGaAs/GaAs quantum dots,” Phys. Rev. Lett. 104, 017402 (2010).
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A. J. Ramsay, T. M. Godden, S. J. Boyle, E. M. Gauger, A. Nazir, B. W. Lovett, A. M. Fox, and M. S. Skolnick, “Phonon-induced Rabi-frequency renormalization of optically driven single InGaAs/GaAs quantum dots,” Phys. Rev. Lett. 105, 177402 (2010).
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Y. J. Wei, Y. M. He, M. C. Chen, Y. N. Hu, Y. He, D. Wu, C. Schneider, M. Kamp, S. Höfling, C. Y. Lu, and J.-W. Pan, “Deterministic and robust generation of single photons from a single quantum dot with 99.5% indistinguishably using adiabatic rapid passage,” Nano Lett. 14, 6515–6519 (2014).
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Y.-J. Wei, Y. He, Y.-M. He, C.-Y. Lu, J.-W. Pan, C. Schneider, M. Kamp, S. Höfling, D. P. S. McCutcheon, and A. Nazir, “Temperature-dependent Mollow triplet spectra from a single quantum dot: Rabi frequency renormalization and sideband linewidth insensitivity,” Phys. Rev. Lett. 113, 097401 (2014).
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A. M. Barth, S. Lüker, A. Vagov, D. E. Reiter, T. Kuhn, and V. M. Axt, “Fast and selective phonon-assisted state preparation of a quantum dot by adiabatic undressing,” Phys. Rev. B, arXiv:1601.07886 (to be published).

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T. M. Godden, J. H. Quilter, A. J. Ramsay, Y. Wu, P. Brereton, S. J. Boyle, I. J. Luxmoore, J. Puebla-Nunez, A. M. Fox, and M. S. Skolnick, “Coherent optical control of the spin of a single hole in an InAs/GaAs quantum dot,” Phys. Rev. Lett. 108, 017402 (2012).
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F. Liu, L. M. P. Martins, A. J. Brash, A. M. Barth, J. H. Quilter, V. M. Axt, M. S. Skolnick, and A. M. Fox, “Ultrafast depopulation of a quantum dot by LA-phonon-assisted stimulated emission,” Phys. Rev. B 93, 161407(R) (2016).

Martins, L. M. P. P.

A. J. Brash, L. M. P. P. Martins, F. Liu, J. H. Quilter, A. J. Ramsay, M. S. Skolnick, and A. M. Fox, “High-fidelity initialization of long-lived quantum dot hole spin qubits by reduced fine-structure splitting,” Phys. Rev. B 92, 121301 (2015).
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R. Mathew, E. Dilcher, A. Gamouras, A. Ramachandran, H. Y. Shi Yang, S. Freisem, D. Deppe, and K. C. Hall, “Subpicosecond adiabatic rapid passage on a single semiconductor quantum dot: phonon-mediated dephasing in the strong-driving regime,” Phys. Rev. B 90, 035316 (2014).
[Crossref]

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J. Hansom, C. H. H. Schulte, C. Matthiesen, M. J. Stanley, and M. Atatüre, “Frequency stabilization of the zero-phonon line of a quantum dot via phonon-assisted active feedback,” Appl. Phys. Lett. 105, 172107 (2014).
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Y.-J. Wei, Y. He, Y.-M. He, C.-Y. Lu, J.-W. Pan, C. Schneider, M. Kamp, S. Höfling, D. P. S. McCutcheon, and A. Nazir, “Temperature-dependent Mollow triplet spectra from a single quantum dot: Rabi frequency renormalization and sideband linewidth insensitivity,” Phys. Rev. Lett. 113, 097401 (2014).
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D. P. S. McCutcheon and A. Nazir, “Model of the optical emission of a driven semiconductor quantum dot: phonon-enhanced coherent scattering and off-resonant sideband narrowing,” Phys. Rev. Lett. 110, 217401 (2013).
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D. P. S. McCutcheon and A. Nazir, “Quantum dot Rabi rotations beyond the weak exciton-phonon coupling regime,” New J. Phys. 12, 113042 (2010).
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P. A. Dalgarno, J. M. Smith, J. McFarlane, B. D. Gerardot, K. Karrai, A. Badolato, P. M. Petroff, and R. J. Warburton, “Coulomb interactions in single charged self-assembled quantum dots: radiative lifetime and recombination energy,” Phys. Rev. B 77, 245311 (2008).
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F. Hargart, M. Müller, K. Roy-Choudhury, S. L. Portalupi, C. Schneider, S. Höfling, M. Kamp, S. Hughes, and P. Michler, “Cavity-enhanced simultaneous dressing of quantum dot exciton and biexciton states,” Phys. Rev. B 93, 115308 (2016).
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S. Bounouar, M. Müller, A. M. Barth, M. Glässl, V. M. Axt, and P. Michler, “Phonon-assisted robust and deterministic two-photon biexciton preparation in a quantum dot,” Phys. Rev. B 91, 161302 (2015).
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S. Weiler, A. Ulhaq, S. M. Ulrich, D. Richter, M. Jetter, P. Michler, C. Roy, and S. Hughes, “Phonon-assisted incoherent excitation of a quantum dot and its emission properties,” Phys. Rev. B 86, 241304(R) (2012).
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S. Ates, S. M. Ulrich, A. Ulhaq, S. Reitzenstein, A. Löffler, S. Höfling, A. Forchel, and P. Michler, “Non-resonant dot-cavity coupling and its potential for resonant single-quantum-dot-spectroscopy,” Nat. Photonics 3, 724–728 (2009).
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L. Monniello, C. Tonin, R. Hostein, A. Lemaitre, A. Martinez, V. Voliotis, and R. Grousson, “Excitation-induced dephasing in a resonantly driven InAs/GaAs quantum dot,” Phys. Rev. Lett. 111, 026403 (2013).
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K. Müller, K. A. Fischer, A. Rundquist, C. Dory, K. G. Lagoudakis, T. Sarmiento, Y. A. Kelaita, V. Borish, and J. Vučković, “Ultrafast polariton-phonon dynamics of strongly coupled quantum dot-nanocavity systems,” Phys. Rev. X 5, 031006 (2015).

P.-L. Ardelt, L. Hanschke, K. A. Fischer, K. Müller, A. Kleinkauf, M. Koller, A. Bechtold, T. Simmet, J. Wierzbowski, H. Riedl, G. Abstreiter, and J. J. Finley, “Dissipative preparation of the exciton and biexciton in self-assembled quantum dots on picosecond time scales,” Phys. Rev. B 90, 241404(R) (2014).
[Crossref]

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F. Hargart, M. Müller, K. Roy-Choudhury, S. L. Portalupi, C. Schneider, S. Höfling, M. Kamp, S. Hughes, and P. Michler, “Cavity-enhanced simultaneous dressing of quantum dot exciton and biexciton states,” Phys. Rev. B 93, 115308 (2016).
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S. Bounouar, M. Müller, A. M. Barth, M. Glässl, V. M. Axt, and P. Michler, “Phonon-assisted robust and deterministic two-photon biexciton preparation in a quantum dot,” Phys. Rev. B 91, 161302 (2015).
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[Crossref]

D. P. S. McCutcheon and A. Nazir, “Model of the optical emission of a driven semiconductor quantum dot: phonon-enhanced coherent scattering and off-resonant sideband narrowing,” Phys. Rev. Lett. 110, 217401 (2013).
[Crossref]

A. J. Ramsay, T. M. Godden, S. J. Boyle, E. M. Gauger, A. Nazir, B. W. Lovett, A. V. Gopal, A. M. Fox, and M. S. Skolnick, “Effect of detuning on the phonon induced dephasing of optically driven InGaAs/GaAs quantum dots,” J. Appl. Phys. 109, 102415 (2011).
[Crossref]

A. J. Ramsay, A. V. Gopal, E. M. Gauger, A. Nazir, B. W. Lovett, A. M. Fox, and M. S. Skolnick, “Damping of exciton Rabi rotations by acoustic phonons in optically excited InGaAs/GaAs quantum dots,” Phys. Rev. Lett. 104, 017402 (2010).
[Crossref]

D. P. S. McCutcheon and A. Nazir, “Quantum dot Rabi rotations beyond the weak exciton-phonon coupling regime,” New J. Phys. 12, 113042 (2010).
[Crossref]

A. J. Ramsay, T. M. Godden, S. J. Boyle, E. M. Gauger, A. Nazir, B. W. Lovett, A. M. Fox, and M. S. Skolnick, “Phonon-induced Rabi-frequency renormalization of optically driven single InGaAs/GaAs quantum dots,” Phys. Rev. Lett. 105, 177402 (2010).
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P. G. Eliseev, H. Li, A. Stintz, G. T. Liu, T. C. Newell, K. J. Malloy, and L. F. Lester, “Transition dipole moment of InAs/InGaAs quantum dots from experiments on ultralow-threshold laser diodes,” Appl. Phys. Lett. 77, 262–264 (2000).
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P. Borri, W. Langbein, S. Schneider, U. Woggon, R. L. Sellin, D. Ouyang, and D. Bimberg, “Ultralong dephasing time in InGaAs quantum dots,” Phys. Rev. Lett. 87, 157401 (2001).
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Y.-J. Wei, Y. He, Y.-M. He, C.-Y. Lu, J.-W. Pan, C. Schneider, M. Kamp, S. Höfling, D. P. S. McCutcheon, and A. Nazir, “Temperature-dependent Mollow triplet spectra from a single quantum dot: Rabi frequency renormalization and sideband linewidth insensitivity,” Phys. Rev. Lett. 113, 097401 (2014).
[Crossref]

Y. J. Wei, Y. M. He, M. C. Chen, Y. N. Hu, Y. He, D. Wu, C. Schneider, M. Kamp, S. Höfling, C. Y. Lu, and J.-W. Pan, “Deterministic and robust generation of single photons from a single quantum dot with 99.5% indistinguishably using adiabatic rapid passage,” Nano Lett. 14, 6515–6519 (2014).
[Crossref]

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P. A. Dalgarno, J. M. Smith, J. McFarlane, B. D. Gerardot, K. Karrai, A. Badolato, P. M. Petroff, and R. J. Warburton, “Coulomb interactions in single charged self-assembled quantum dots: radiative lifetime and recombination energy,” Phys. Rev. B 77, 245311 (2008).
[Crossref]

Portalupi, S. L.

F. Hargart, M. Müller, K. Roy-Choudhury, S. L. Portalupi, C. Schneider, S. Höfling, M. Kamp, S. Hughes, and P. Michler, “Cavity-enhanced simultaneous dressing of quantum dot exciton and biexciton states,” Phys. Rev. B 93, 115308 (2016).
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S. L. Portalupi, G. Hornecker, V. Giesz, T. Grange, A. Lemaître, J. Demory, I. Sagnes, N. D. Lanzillotti-Kimura, L. Lanco, A. Auffèves, and P. Senellart, “Bright phonon-tuned single-photon source,” Nano Lett. 15, 6290–6294 (2015).
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Puebla-Nunez, J.

T. M. Godden, J. H. Quilter, A. J. Ramsay, Y. Wu, P. Brereton, S. J. Boyle, I. J. Luxmoore, J. Puebla-Nunez, A. M. Fox, and M. S. Skolnick, “Coherent optical control of the spin of a single hole in an InAs/GaAs quantum dot,” Phys. Rev. Lett. 108, 017402 (2012).
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F. Liu, L. M. P. Martins, A. J. Brash, A. M. Barth, J. H. Quilter, V. M. Axt, M. S. Skolnick, and A. M. Fox, “Ultrafast depopulation of a quantum dot by LA-phonon-assisted stimulated emission,” Phys. Rev. B 93, 161407(R) (2016).

A. J. Brash, L. M. P. P. Martins, F. Liu, J. H. Quilter, A. J. Ramsay, M. S. Skolnick, and A. M. Fox, “High-fidelity initialization of long-lived quantum dot hole spin qubits by reduced fine-structure splitting,” Phys. Rev. B 92, 121301 (2015).
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J. H. Quilter, A. J. Brash, F. Liu, M. Glässl, A. M. Barth, V. M. Axt, A. J. Ramsay, M. S. Skolnick, and A. M. Fox, “Phonon-assisted population inversion of a single InGaAs/GaAs quantum dot by pulsed laser excitation,” Phys. Rev. Lett. 114, 137401 (2015).
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R. Mathew, E. Dilcher, A. Gamouras, A. Ramachandran, H. Y. Shi Yang, S. Freisem, D. Deppe, and K. C. Hall, “Subpicosecond adiabatic rapid passage on a single semiconductor quantum dot: phonon-mediated dephasing in the strong-driving regime,” Phys. Rev. B 90, 035316 (2014).
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A. J. Brash, L. M. P. P. Martins, F. Liu, J. H. Quilter, A. J. Ramsay, M. S. Skolnick, and A. M. Fox, “High-fidelity initialization of long-lived quantum dot hole spin qubits by reduced fine-structure splitting,” Phys. Rev. B 92, 121301 (2015).
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J. H. Quilter, A. J. Brash, F. Liu, M. Glässl, A. M. Barth, V. M. Axt, A. J. Ramsay, M. S. Skolnick, and A. M. Fox, “Phonon-assisted population inversion of a single InGaAs/GaAs quantum dot by pulsed laser excitation,” Phys. Rev. Lett. 114, 137401 (2015).
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[Crossref]

A. J. Ramsay, T. M. Godden, S. J. Boyle, E. M. Gauger, A. Nazir, B. W. Lovett, A. V. Gopal, A. M. Fox, and M. S. Skolnick, “Effect of detuning on the phonon induced dephasing of optically driven InGaAs/GaAs quantum dots,” J. Appl. Phys. 109, 102415 (2011).
[Crossref]

A. J. Ramsay, A. V. Gopal, E. M. Gauger, A. Nazir, B. W. Lovett, A. M. Fox, and M. S. Skolnick, “Damping of exciton Rabi rotations by acoustic phonons in optically excited InGaAs/GaAs quantum dots,” Phys. Rev. Lett. 104, 017402 (2010).
[Crossref]

A. J. Ramsay, T. M. Godden, S. J. Boyle, E. M. Gauger, A. Nazir, B. W. Lovett, A. M. Fox, and M. S. Skolnick, “Phonon-induced Rabi-frequency renormalization of optically driven single InGaAs/GaAs quantum dots,” Phys. Rev. Lett. 105, 177402 (2010).
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S. J. Boyle, A. J. Ramsay, A. M. Fox, M. S. Skolnick, A. P. Heberle, and M. Hopkinson, “Beating of exciton dressed states in a single semiconductor InGaAs/GaAs quantum dot,” Phys. Rev. Lett. 102, 207401 (2009).
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S. J. Boyle, A. J. Ramsay, F. Bello, H. Y. Liu, M. Hopkinson, A. M. Fox, and M. S. Skolnick, “Two-qubit conditional quantum-logic operation in a single self-assembled quantum dot,” Phys. Rev. B 78, 075301 (2008).
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T. Volz, A. Reinhard, M. Winger, A. Badolato, K. J. Hennessy, E. L. Hu, and A. Imamoglu, “Ultrafast all-optical switching by single photons,” Nat. Photonics 6, 607–611 (2012).
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A. M. Barth, S. Lüker, A. Vagov, D. E. Reiter, T. Kuhn, and V. M. Axt, “Fast and selective phonon-assisted state preparation of a quantum dot by adiabatic undressing,” Phys. Rev. B, arXiv:1601.07886 (to be published).

Reitzenstein, S.

S. Ates, S. M. Ulrich, A. Ulhaq, S. Reitzenstein, A. Löffler, S. Höfling, A. Forchel, and P. Michler, “Non-resonant dot-cavity coupling and its potential for resonant single-quantum-dot-spectroscopy,” Nat. Photonics 3, 724–728 (2009).
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S. Weiler, A. Ulhaq, S. M. Ulrich, D. Richter, M. Jetter, P. Michler, C. Roy, and S. Hughes, “Phonon-assisted incoherent excitation of a quantum dot and its emission properties,” Phys. Rev. B 86, 241304(R) (2012).
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P.-L. Ardelt, L. Hanschke, K. A. Fischer, K. Müller, A. Kleinkauf, M. Koller, A. Bechtold, T. Simmet, J. Wierzbowski, H. Riedl, G. Abstreiter, and J. J. Finley, “Dissipative preparation of the exciton and biexciton in self-assembled quantum dots on picosecond time scales,” Phys. Rev. B 90, 241404(R) (2014).
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F. Hargart, M. Müller, K. Roy-Choudhury, S. L. Portalupi, C. Schneider, S. Höfling, M. Kamp, S. Hughes, and P. Michler, “Cavity-enhanced simultaneous dressing of quantum dot exciton and biexciton states,” Phys. Rev. B 93, 115308 (2016).
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K. Müller, K. A. Fischer, A. Rundquist, C. Dory, K. G. Lagoudakis, T. Sarmiento, Y. A. Kelaita, V. Borish, and J. Vučković, “Ultrafast polariton-phonon dynamics of strongly coupled quantum dot-nanocavity systems,” Phys. Rev. X 5, 031006 (2015).

Sagnes, I.

S. L. Portalupi, G. Hornecker, V. Giesz, T. Grange, A. Lemaître, J. Demory, I. Sagnes, N. D. Lanzillotti-Kimura, L. Lanco, A. Auffèves, and P. Senellart, “Bright phonon-tuned single-photon source,” Nano Lett. 15, 6290–6294 (2015).
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K. Müller, K. A. Fischer, A. Rundquist, C. Dory, K. G. Lagoudakis, T. Sarmiento, Y. A. Kelaita, V. Borish, and J. Vučković, “Ultrafast polariton-phonon dynamics of strongly coupled quantum dot-nanocavity systems,” Phys. Rev. X 5, 031006 (2015).

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R. Schirhagl, K. Chang, M. Loretz, and C. L. Degen, “Nitrogen-vacancy centers in diamond: nanoscale sensors for physics and biology,” Ann. Rev. Phys. Chem. 65, 83–105 (2014).
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F. Hargart, M. Müller, K. Roy-Choudhury, S. L. Portalupi, C. Schneider, S. Höfling, M. Kamp, S. Hughes, and P. Michler, “Cavity-enhanced simultaneous dressing of quantum dot exciton and biexciton states,” Phys. Rev. B 93, 115308 (2016).
[Crossref]

Y. J. Wei, Y. M. He, M. C. Chen, Y. N. Hu, Y. He, D. Wu, C. Schneider, M. Kamp, S. Höfling, C. Y. Lu, and J.-W. Pan, “Deterministic and robust generation of single photons from a single quantum dot with 99.5% indistinguishably using adiabatic rapid passage,” Nano Lett. 14, 6515–6519 (2014).
[Crossref]

Y.-J. Wei, Y. He, Y.-M. He, C.-Y. Lu, J.-W. Pan, C. Schneider, M. Kamp, S. Höfling, D. P. S. McCutcheon, and A. Nazir, “Temperature-dependent Mollow triplet spectra from a single quantum dot: Rabi frequency renormalization and sideband linewidth insensitivity,” Phys. Rev. Lett. 113, 097401 (2014).
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P. Borri, W. Langbein, S. Schneider, U. Woggon, R. L. Sellin, D. Ouyang, and D. Bimberg, “Ultralong dephasing time in InGaAs quantum dots,” Phys. Rev. Lett. 87, 157401 (2001).
[Crossref]

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J. Hansom, C. H. H. Schulte, C. Matthiesen, M. J. Stanley, and M. Atatüre, “Frequency stabilization of the zero-phonon line of a quantum dot via phonon-assisted active feedback,” Appl. Phys. Lett. 105, 172107 (2014).
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P. Borri, W. Langbein, S. Schneider, U. Woggon, R. L. Sellin, D. Ouyang, and D. Bimberg, “Ultralong dephasing time in InGaAs quantum dots,” Phys. Rev. Lett. 87, 157401 (2001).
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S. L. Portalupi, G. Hornecker, V. Giesz, T. Grange, A. Lemaître, J. Demory, I. Sagnes, N. D. Lanzillotti-Kimura, L. Lanco, A. Auffèves, and P. Senellart, “Bright phonon-tuned single-photon source,” Nano Lett. 15, 6290–6294 (2015).
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Shi Yang, H. Y.

R. Mathew, E. Dilcher, A. Gamouras, A. Ramachandran, H. Y. Shi Yang, S. Freisem, D. Deppe, and K. C. Hall, “Subpicosecond adiabatic rapid passage on a single semiconductor quantum dot: phonon-mediated dephasing in the strong-driving regime,” Phys. Rev. B 90, 035316 (2014).
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D. Heinze, D. Breddermann, A. Zrenner, and S. Schumacher, “A quantum dot single-photon source with on-the-fly all-optical polarization control and timed emission,” Nat. Commun. 6, 8473 (2015).
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K. H. Madsen, S. Ates, J. Liu, A. Javadi, S. M. Albrecht, I. Yeo, S. Stobbe, and P. Lodahl, “Efficient out-coupling of high-purity single photons from a coherent quantum dot in a photonic-crystal cavity,” Phys. Rev. B 90, 155303 (2014).
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S. J. Boyle, A. J. Ramsay, F. Bello, H. Y. Liu, M. Hopkinson, A. M. Fox, and M. S. Skolnick, “Two-qubit conditional quantum-logic operation in a single self-assembled quantum dot,” Phys. Rev. B 78, 075301 (2008).
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A. J. Brash, L. M. P. P. Martins, F. Liu, J. H. Quilter, A. J. Ramsay, M. S. Skolnick, and A. M. Fox, “High-fidelity initialization of long-lived quantum dot hole spin qubits by reduced fine-structure splitting,” Phys. Rev. B 92, 121301 (2015).
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A. J. Ramsay, A. V. Gopal, E. M. Gauger, A. Nazir, B. W. Lovett, A. M. Fox, and M. S. Skolnick, “Damping of exciton Rabi rotations by acoustic phonons in optically excited InGaAs/GaAs quantum dots,” Phys. Rev. Lett. 104, 017402 (2010).
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T. M. Godden, J. H. Quilter, A. J. Ramsay, Y. Wu, P. Brereton, S. J. Boyle, I. J. Luxmoore, J. Puebla-Nunez, A. M. Fox, and M. S. Skolnick, “Coherent optical control of the spin of a single hole in an InAs/GaAs quantum dot,” Phys. Rev. Lett. 108, 017402 (2012).
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P. Borri, W. Langbein, S. Schneider, U. Woggon, R. L. Sellin, D. Ouyang, and D. Bimberg, “Ultralong dephasing time in InGaAs quantum dots,” Phys. Rev. Lett. 87, 157401 (2001).
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Figures (8)

Fig. 1.
Fig. 1. Calculation of the dynamics of the dressed states when excited with a 16.8 ps laser pulse centered at t = 0 with Δ = + 1    meV and Θ = 8.5 π . (a) Energies of the dressed states (green lines) | α and | β plotted against time. At t , the states are split by the laser detuning Δ . During the passage of the pulse, the states are admixed and the splitting becomes Λ as shown by the shift centered at t = 0 . This enables relaxation from | α to | β (blue arrows) by emission of an LA phonon with energy Λ . (b) Plot of the admixing angle θ (black line) and the population of the dressed state | β (blue line) against time. θ also follows the envelope of the laser pulse and, as expected, relaxation into | β occurs only when the states are admixed.
Fig. 2.
Fig. 2. (a) Illustration of the energies of the dressed states | α and | β plotted against detuning Δ at a fixed time. The bare QD states in the frame of the laser are plotted for reference as dotted black lines. At Δ = 0 , the states anti-cross with a splitting of Ω R . It can be seen that | α is dominated by the ground state at Δ > 0 , leading to phonon-assisted excitation of the exciton. Conversely, | α is primarily excitonic in character at Δ < 0 , and thus phonon-assisted de-excitation of the exciton occurs. The blue arrows illustrate the relaxation process corresponding to the emission of an LA phonon, while the red arrows show the competing phonon absorption process. (b)–(e) Phenomenological energy level diagrams of the phonon emission and absorption processes for both positive and negative detunings. For simplicity, the phonon relaxation is incorporated as a virtual state (dashed lines).
Fig. 3.
Fig. 3. Plot of the exciton–phonon interaction strength J ( ω ) as determined by fitting data measured in Ref. [24]. The interaction strength peaks at a cutoff of around 2 meV and rolls off rapidly beyond this.
Fig. 4.
Fig. 4. Experimental arrangement. A femtosecond pulsed laser beam is split into two paths. The wavelength, FWHM, arrival time, and polarization of the two pulses are controlled independently by the pulse shapers, delay stage, and wave plates (WP). Finally the two beams are combined and sent to the sample, which is kept in a variable temperature liquid-He cryostat. The exciton created by the laser pulse is measured by detecting the PC generated from the QD.
Fig. 5.
Fig. 5. Comparison of Ramsey-like fringe data on the exciton for pumping in the phonon sideband (red) and at the exciton (black) at T = 4.2    K . In both cases, the second π / 2 -pulse is resonant with the exciton. The pulse area Θ of the + 1    meV detuned pump pulse is set to be 8.4 π to generate C X = 0.5 . The dashed line is a guide to the eye.
Fig. 6.
Fig. 6. Demonstration of the spin selectivity of the LAPSE process. (a), (b) Differential PC spectra Δ P C were obtained by preparing an exciton in the QD using a circularly polarized π pulse and then measuring the PC as a function of a co-/cross-polarized LAPSE pulse. To isolate the PC signal of the QD under study from other QDs in the same sample, a reference spectrum measured with only a redshifted laser pulse is subtracted. The pulse area Θ of the redshifted laser pulse is (black) π or (red) 7.35 π . The delay time between the π pulse and the redshifted pulse is 17 ps. X X : biexciton.
Fig. 7.
Fig. 7. (a) Exciton population versus laser detuning ( Δ ) at 15 K (red triangles) compared to 4.2 K (black circles) for excitation with pulse area Θ = 4.4 π . The dashed line indicates a detuning of Δ = + 0.83    meV . (b) Calculated variation of the exciton population versus pulse area ( Θ ) for T = 4.2    K (black), T = 15    K (red), and T = 25    K (blue) for positive detuning of Δ = + 0.83    meV . The dashed line shows Θ = 4.4 π .
Fig. 8.
Fig. 8. (a) PC signal measured with positively and negatively detuned control pulses as a function of the delay time τ delay = t OFF t ON , where t OFF and t ON are the arrival time of the de-excitation and excitation pulses, respectively. Δ = ± 0.7    meV ; Θ = 5.25 π ; FWHM = 0.42    meV ; Pulse duration = 8    ps . Inset: pulse sequence. (b) Exciton population calculated in the two-color pump–probe measurement using parameters similar to those of Fig. 8(a). Δ = ± 0.7    meV ; Θ = 5.25 π ; pulse duration = 10    ps .

Equations (6)

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Θ = + Ω R ( t ) d t ,
| α = sin ( θ ) | 0 + cos ( θ ) | X
| β = cos ( θ ) | 0 sin ( θ ) | X ,
tan ( 2 θ ) = Ω R / Δ , 0 2 θ 180 ° .
E ± = 2 ( Δ ± Λ ( t ) ) ,
Λ ( t ) = Ω R ( t ) 2 + Δ 2 .

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