Abstract
We describe a detailed photon correlation Fourier spectroscopy (PCFS) study of a single nanocrystal at . PCFS provides the temporal and spectral resolution that is necessary for such a fast spectrally diffusing emitter. In the emitter spectrum, we distinguish a main zero-phonon line, the one- and two-longitudinal-optical-phonon replica, and the longitudinal-acoustic-phonon pedestal. We determine the spectral diffusion amplitude as a function of time for timescales from and propose an interpretation for the two observed regimes.
© 2009 Optical Society of America
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