Abstract

We present nanosecond hole-burning experiments for CdSxSe1−x and CdSe quantum dots grown in a glass matrix; we compare the results for different precipitation stages. For the first time to our knowledge a drastic sharpening of the spectral holes with a half-width as low as 10 meV has been found to be typical for the samples prepared in the nucleation and the normal growth stages, whereas structures grown in the coalescent stage show only broadband nonlinear absorption. The spectral width of the holes is highly sensitive to the illumination history, particularly in the case of small-size quantum dots. A coexistence of quantum dots from the coalescent and the noncoalescent growth regimes results in a structured nonlinear absorption spectrum from the superposition of the corresponding broadband and narrow-line nonlinear spectra; thus the actual electronic-level structure can be completely masked. The differences in the linewidth are attributed to different mechanisms of surface construction or reconstruction during the growth process or after strong laser exposure, leading to different surface properties such as localized states or spatial charge distributions, which in turn give rise to different mechanisms of line broadening.

© 1993 Optical Society of America

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  19. P. Roussignol, D. Ricard, J. Lukasik, and C. Flytzanis, J. Opt. Soc. Am. B 4, 5 (1987).
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  21. L. Banyai, P. Gilliot, Y. Z. Hu, and S. W. Koch, Phys. Rev. B 45, 14136 (1992).
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  22. Al. L. Efros, Superlattices Microstruct. 11, 167 (1992).
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  25. L. G. Zimin, S. V. Gaponenko, and V. Yu. Lebed, Phys. Status Solidi B 150, 653 (1988).
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  30. A. P. Alivisatos, A. L. Harris, N. J. Levinos, M. L. Steigerwald, and L. E. Brus, J. Chem. Phys. 89, 4001 (1988).
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  31. M. G. Bawendi, P. J. Caroll, W. L. Wilson, and L. E. Brus, J. Chem. Phys. 96, 946 (1992).
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  32. Y. Wang, N. Herron, W. Mahler, and A. Suna, J. Opt. Soc. Am. B 6, 808 (1989).
    [Crossref]
  33. U. Woggon, M. Müller, U. Lembke, I. Rückmann, and J. Cesnulevicius, Superlattices Microstruct. 9, 245 (1991).
    [Crossref]
  34. A. Uhrig, A. Wörner, C. Klingshirn, L. Banyai, S. Gaponenko, I. Lacis, N. Neuroth, B. Speith, and K. Remitz, J. Cryst. Growth 117, 598 (1992).
    [Crossref]
  35. Al. L. Efros and A. L. Efros, Sov. Phys. Semicond. 16, 772 (1982).
  36. I. M. Lifshiz and V. V. Slesov, Zh. Eksp. Teor. Fiz. 35, 479 (1958).
  37. S. W. Koch, Y. Z. Hu, B. Fluegel, and N. Peyghambarian, J. Cryst. Growth 117, 592 (1992).
    [Crossref]
  38. A. I. Ekimov, F. Hache, M. C. Schanne-Klein, D. Ricard, C. Flytzanis, I. A. Kudryavtsev, T. V. Yazeva, A. V. Rodina, and Al. L. Efros, J. Opt. Soc. Am. B 10, 100 (1993).
    [Crossref]
  39. Jian-Bai Xia, Phys. Rev. B 40, 8500 (1989).
    [Crossref]
  40. G. B. Grygoryan, E. M. Kazaryan, Al. L. Efros, and T. V. Yazeva, Sov. Phys. Solid State 32, 1031 (1990).
  41. Y. Z. Hu, M. Lindberg, and S. W. Koch, Phys. Rev. B 42, 1713 (1990).
    [Crossref]
  42. S. H. Park, R. A. Morgan, Y. Z. Hu, M. Lindberg, S. W. Koch, and N. Peyghambarian, J. Opt. Soc. Am. B 7, 2097 (1990).
    [Crossref]

1993 (1)

1992 (9)

M. P. A. Müller, U. Lembke, U. Woggon, and I. Rückmann, J. Non-Cryst. Solids 144, 240 (1992).
[Crossref]

L. Banyai, P. Gilliot, Y. Z. Hu, and S. W. Koch, Phys. Rev. B 45, 14136 (1992).
[Crossref]

Al. L. Efros, Superlattices Microstruct. 11, 167 (1992).
[Crossref]

S. Nomura and T. Kobayashi, Phys. Rev. B 45, 1305 (1992).
[Crossref]

U. Woggon, I. Rückmann, J. Kornack, M. Müller, J. Cesnulevicius, M. Petrauskas, and J. Kolenda, J. Cryst. Growth 117, 608 (1992).
[Crossref]

M. G. Bawendi, P. J. Caroll, W. L. Wilson, and L. E. Brus, J. Chem. Phys. 96, 946 (1992).
[Crossref]

A. Uhrig, A. Wörner, C. Klingshirn, L. Banyai, S. Gaponenko, I. Lacis, N. Neuroth, B. Speith, and K. Remitz, J. Cryst. Growth 117, 598 (1992).
[Crossref]

S. W. Koch, Y. Z. Hu, B. Fluegel, and N. Peyghambarian, J. Cryst. Growth 117, 592 (1992).
[Crossref]

V. Esch, K. Kang, B. Fluegel, Y. Z. Hu, G. Khitrova, L. C. Liu, and L. C. Risbud, J. Nonlin. Opt. Phys. 1, 25 (1992).
[Crossref]

1991 (8)

U. Woggon, M. Müller, U. Lembke, I. Rückmann, and J. Cesnulevicius, Superlattices Microstruct. 9, 245 (1991).
[Crossref]

T. Yanagawa, H. Nakano, and Y. Sasaki, Appl. Phys. Lett. 59, 1690 (1991).
[Crossref]

J. Malhotra, D. J. Hagan, and B. G. Potter, J. Opt. Soc. Am. B 7, 1531 (1991).
[Crossref]

A. Uhrig, L. Banyai, S. Gaponenko, A. Wörner, N. Neuroth, and C. Klingshirn, Z. Phys. D 20, 345 (1991).
[Crossref]

Ch. Spiegelberg, F. Henneberger, and J. Puls, Superlattices Microstruct. 9, 487 (1991).
[Crossref]

A. I. Ekimov, Phys. Scr. T39, 217 (1991).
[Crossref]

L. E. Brus, Appl. Phys. A 53, 465 (1991).
[Crossref]

F. Hache, M. C. Klein, D. Ricard, and C. Flytzanis, J. Opt. Soc. Am. B 8, 1802 (1991).
[Crossref]

1990 (8)

L. C. Liu and S. H. Risbud, J. Appl. Phys. 68, 28 (1990).
[Crossref]

A. R. Kottan, R. Hull, R. L. Opila, M. G. Bawendi, M. L. Steigerwald, P. J. Caroll, and L. E. Brus, J. Am. Chem. Soc. 112, 1327 (1990).
[Crossref]

A. Uhrig, L. Banyai, Y. Z. Hu, S. W. Koch, C. Klingshirn, and N. Neuroth, Z. Phys. B 81, 385 (1990).
[Crossref]

G. B. Grygoryan, E. M. Kazaryan, Al. L. Efros, and T. V. Yazeva, Sov. Phys. Solid State 32, 1031 (1990).

Y. Z. Hu, M. Lindberg, and S. W. Koch, Phys. Rev. B 42, 1713 (1990).
[Crossref]

M. Tomita and M. Matsuoka, J. Opt. Soc. Am. B 7, 1198 (1990).
[Crossref]

S. H. Park, R. A. Morgan, Y. Z. Hu, M. Lindberg, S. W. Koch, and N. Peyghambarian, J. Opt. Soc. Am. B 7, 2097 (1990).
[Crossref]

S. H. Park, R. A. Morgan, Y. Z. Hu, M. Lindberg, S. W. Koch, and N. Peyghambarian, J. Opt. Soc. Am. B 7, 2097 (1990).
[Crossref]

1989 (7)

Y. Wang, N. Herron, W. Mahler, and A. Suna, J. Opt. Soc. Am. B 6, 808 (1989).
[Crossref]

K. W. DeLong, A. Gabel, C. T. Seaton, and G. I. Stegeman, J. Opt. Soc. Am. B 6, 1306 (1989).
[Crossref]

P. Roussignol, D. Ricard, C. Flytzanis, and N. Neuroth, Phys. Rev. Lett. 62, 312 (1989).
[Crossref] [PubMed]

Jian-Bai Xia, Phys. Rev. B 40, 8500 (1989).
[Crossref]

M. L. Steigerwald and L. E. Brus, Annu. Rev. Mater. Sci. 19, 471 (1989).
[Crossref]

B. van Wonterghem, S. M. Saltiel, T. E. Dutton, and P. M. Rentzepis, J. Appl. Phys. 66, 4935 (1989).
[Crossref]

F. Yan and J. M. Parker, J. Non-Cryst. Solids 112, 277 (1989).
[Crossref]

1988 (3)

B. G. Potter and J. H. Simmons, Phys. Rev. B 37, 10838 (1988).
[Crossref]

L. G. Zimin, S. V. Gaponenko, and V. Yu. Lebed, Phys. Status Solidi B 150, 653 (1988).
[Crossref]

A. P. Alivisatos, A. L. Harris, N. J. Levinos, M. L. Steigerwald, and L. E. Brus, J. Chem. Phys. 89, 4001 (1988).
[Crossref]

1987 (3)

N. F. Borelli, D. W. Hall, H. J. Holland, and D. W. Smith, J. Appl. Phys. 61, 5399 (1987).
[Crossref]

S. Schmitt-Rink, D. A. B. Miller, and D. S. Chemla, Phys. Rev. B 35, 8113 (1987).
[Crossref]

P. Roussignol, D. Ricard, J. Lukasik, and C. Flytzanis, J. Opt. Soc. Am. B 4, 5 (1987).
[Crossref]

1982 (1)

Al. L. Efros and A. L. Efros, Sov. Phys. Semicond. 16, 772 (1982).

1958 (1)

I. M. Lifshiz and V. V. Slesov, Zh. Eksp. Teor. Fiz. 35, 479 (1958).

Alivisatos, A. P.

A. P. Alivisatos, A. L. Harris, N. J. Levinos, M. L. Steigerwald, and L. E. Brus, J. Chem. Phys. 89, 4001 (1988).
[Crossref]

Banyai, L.

A. Uhrig, A. Wörner, C. Klingshirn, L. Banyai, S. Gaponenko, I. Lacis, N. Neuroth, B. Speith, and K. Remitz, J. Cryst. Growth 117, 598 (1992).
[Crossref]

L. Banyai, P. Gilliot, Y. Z. Hu, and S. W. Koch, Phys. Rev. B 45, 14136 (1992).
[Crossref]

A. Uhrig, L. Banyai, S. Gaponenko, A. Wörner, N. Neuroth, and C. Klingshirn, Z. Phys. D 20, 345 (1991).
[Crossref]

A. Uhrig, L. Banyai, Y. Z. Hu, S. W. Koch, C. Klingshirn, and N. Neuroth, Z. Phys. B 81, 385 (1990).
[Crossref]

Bawendi, M. G.

M. G. Bawendi, P. J. Caroll, W. L. Wilson, and L. E. Brus, J. Chem. Phys. 96, 946 (1992).
[Crossref]

A. R. Kottan, R. Hull, R. L. Opila, M. G. Bawendi, M. L. Steigerwald, P. J. Caroll, and L. E. Brus, J. Am. Chem. Soc. 112, 1327 (1990).
[Crossref]

Borelli, N. F.

N. F. Borelli, D. W. Hall, H. J. Holland, and D. W. Smith, J. Appl. Phys. 61, 5399 (1987).
[Crossref]

Brus, L. E.

M. G. Bawendi, P. J. Caroll, W. L. Wilson, and L. E. Brus, J. Chem. Phys. 96, 946 (1992).
[Crossref]

L. E. Brus, Appl. Phys. A 53, 465 (1991).
[Crossref]

A. R. Kottan, R. Hull, R. L. Opila, M. G. Bawendi, M. L. Steigerwald, P. J. Caroll, and L. E. Brus, J. Am. Chem. Soc. 112, 1327 (1990).
[Crossref]

M. L. Steigerwald and L. E. Brus, Annu. Rev. Mater. Sci. 19, 471 (1989).
[Crossref]

A. P. Alivisatos, A. L. Harris, N. J. Levinos, M. L. Steigerwald, and L. E. Brus, J. Chem. Phys. 89, 4001 (1988).
[Crossref]

Caroll, P. J.

M. G. Bawendi, P. J. Caroll, W. L. Wilson, and L. E. Brus, J. Chem. Phys. 96, 946 (1992).
[Crossref]

A. R. Kottan, R. Hull, R. L. Opila, M. G. Bawendi, M. L. Steigerwald, P. J. Caroll, and L. E. Brus, J. Am. Chem. Soc. 112, 1327 (1990).
[Crossref]

Cesnulevicius, J.

U. Woggon, I. Rückmann, J. Kornack, M. Müller, J. Cesnulevicius, M. Petrauskas, and J. Kolenda, J. Cryst. Growth 117, 608 (1992).
[Crossref]

U. Woggon, M. Müller, U. Lembke, I. Rückmann, and J. Cesnulevicius, Superlattices Microstruct. 9, 245 (1991).
[Crossref]

Chemla, D. S.

S. Schmitt-Rink, D. A. B. Miller, and D. S. Chemla, Phys. Rev. B 35, 8113 (1987).
[Crossref]

DeLong, K. W.

Dutton, T. E.

B. van Wonterghem, S. M. Saltiel, T. E. Dutton, and P. M. Rentzepis, J. Appl. Phys. 66, 4935 (1989).
[Crossref]

Efros, A. L.

Al. L. Efros and A. L. Efros, Sov. Phys. Semicond. 16, 772 (1982).

Efros, Al. L.

A. I. Ekimov, F. Hache, M. C. Schanne-Klein, D. Ricard, C. Flytzanis, I. A. Kudryavtsev, T. V. Yazeva, A. V. Rodina, and Al. L. Efros, J. Opt. Soc. Am. B 10, 100 (1993).
[Crossref]

Al. L. Efros, Superlattices Microstruct. 11, 167 (1992).
[Crossref]

G. B. Grygoryan, E. M. Kazaryan, Al. L. Efros, and T. V. Yazeva, Sov. Phys. Solid State 32, 1031 (1990).

Al. L. Efros and A. L. Efros, Sov. Phys. Semicond. 16, 772 (1982).

Ekimov, A. I.

Esch, V.

V. Esch, K. Kang, B. Fluegel, Y. Z. Hu, G. Khitrova, L. C. Liu, and L. C. Risbud, J. Nonlin. Opt. Phys. 1, 25 (1992).
[Crossref]

Fluegel, B.

V. Esch, K. Kang, B. Fluegel, Y. Z. Hu, G. Khitrova, L. C. Liu, and L. C. Risbud, J. Nonlin. Opt. Phys. 1, 25 (1992).
[Crossref]

S. W. Koch, Y. Z. Hu, B. Fluegel, and N. Peyghambarian, J. Cryst. Growth 117, 592 (1992).
[Crossref]

Flytzanis, C.

Gabel, A.

Gaponenko, S.

A. Uhrig, A. Wörner, C. Klingshirn, L. Banyai, S. Gaponenko, I. Lacis, N. Neuroth, B. Speith, and K. Remitz, J. Cryst. Growth 117, 598 (1992).
[Crossref]

A. Uhrig, L. Banyai, S. Gaponenko, A. Wörner, N. Neuroth, and C. Klingshirn, Z. Phys. D 20, 345 (1991).
[Crossref]

Gaponenko, S. V.

L. G. Zimin, S. V. Gaponenko, and V. Yu. Lebed, Phys. Status Solidi B 150, 653 (1988).
[Crossref]

Gilliot, P.

L. Banyai, P. Gilliot, Y. Z. Hu, and S. W. Koch, Phys. Rev. B 45, 14136 (1992).
[Crossref]

Grygoryan, G. B.

G. B. Grygoryan, E. M. Kazaryan, Al. L. Efros, and T. V. Yazeva, Sov. Phys. Solid State 32, 1031 (1990).

Hache, F.

Hagan, D. J.

J. Malhotra, D. J. Hagan, and B. G. Potter, J. Opt. Soc. Am. B 7, 1531 (1991).
[Crossref]

Hall, D. W.

N. F. Borelli, D. W. Hall, H. J. Holland, and D. W. Smith, J. Appl. Phys. 61, 5399 (1987).
[Crossref]

Harris, A. L.

A. P. Alivisatos, A. L. Harris, N. J. Levinos, M. L. Steigerwald, and L. E. Brus, J. Chem. Phys. 89, 4001 (1988).
[Crossref]

Henneberger, F.

Ch. Spiegelberg, F. Henneberger, and J. Puls, Superlattices Microstruct. 9, 487 (1991).
[Crossref]

Herron, N.

Holland, H. J.

N. F. Borelli, D. W. Hall, H. J. Holland, and D. W. Smith, J. Appl. Phys. 61, 5399 (1987).
[Crossref]

Hu, Y. Z.

L. Banyai, P. Gilliot, Y. Z. Hu, and S. W. Koch, Phys. Rev. B 45, 14136 (1992).
[Crossref]

V. Esch, K. Kang, B. Fluegel, Y. Z. Hu, G. Khitrova, L. C. Liu, and L. C. Risbud, J. Nonlin. Opt. Phys. 1, 25 (1992).
[Crossref]

S. W. Koch, Y. Z. Hu, B. Fluegel, and N. Peyghambarian, J. Cryst. Growth 117, 592 (1992).
[Crossref]

Y. Z. Hu, M. Lindberg, and S. W. Koch, Phys. Rev. B 42, 1713 (1990).
[Crossref]

S. H. Park, R. A. Morgan, Y. Z. Hu, M. Lindberg, S. W. Koch, and N. Peyghambarian, J. Opt. Soc. Am. B 7, 2097 (1990).
[Crossref]

S. H. Park, R. A. Morgan, Y. Z. Hu, M. Lindberg, S. W. Koch, and N. Peyghambarian, J. Opt. Soc. Am. B 7, 2097 (1990).
[Crossref]

A. Uhrig, L. Banyai, Y. Z. Hu, S. W. Koch, C. Klingshirn, and N. Neuroth, Z. Phys. B 81, 385 (1990).
[Crossref]

Hull, R.

A. R. Kottan, R. Hull, R. L. Opila, M. G. Bawendi, M. L. Steigerwald, P. J. Caroll, and L. E. Brus, J. Am. Chem. Soc. 112, 1327 (1990).
[Crossref]

Kang, K.

V. Esch, K. Kang, B. Fluegel, Y. Z. Hu, G. Khitrova, L. C. Liu, and L. C. Risbud, J. Nonlin. Opt. Phys. 1, 25 (1992).
[Crossref]

Kazaryan, E. M.

G. B. Grygoryan, E. M. Kazaryan, Al. L. Efros, and T. V. Yazeva, Sov. Phys. Solid State 32, 1031 (1990).

Khitrova, G.

V. Esch, K. Kang, B. Fluegel, Y. Z. Hu, G. Khitrova, L. C. Liu, and L. C. Risbud, J. Nonlin. Opt. Phys. 1, 25 (1992).
[Crossref]

Klein, M. C.

Klingshirn, C.

A. Uhrig, A. Wörner, C. Klingshirn, L. Banyai, S. Gaponenko, I. Lacis, N. Neuroth, B. Speith, and K. Remitz, J. Cryst. Growth 117, 598 (1992).
[Crossref]

A. Uhrig, L. Banyai, S. Gaponenko, A. Wörner, N. Neuroth, and C. Klingshirn, Z. Phys. D 20, 345 (1991).
[Crossref]

A. Uhrig, L. Banyai, Y. Z. Hu, S. W. Koch, C. Klingshirn, and N. Neuroth, Z. Phys. B 81, 385 (1990).
[Crossref]

Kobayashi, T.

S. Nomura and T. Kobayashi, Phys. Rev. B 45, 1305 (1992).
[Crossref]

Koch, S. W.

L. Banyai, P. Gilliot, Y. Z. Hu, and S. W. Koch, Phys. Rev. B 45, 14136 (1992).
[Crossref]

S. W. Koch, Y. Z. Hu, B. Fluegel, and N. Peyghambarian, J. Cryst. Growth 117, 592 (1992).
[Crossref]

Y. Z. Hu, M. Lindberg, and S. W. Koch, Phys. Rev. B 42, 1713 (1990).
[Crossref]

S. H. Park, R. A. Morgan, Y. Z. Hu, M. Lindberg, S. W. Koch, and N. Peyghambarian, J. Opt. Soc. Am. B 7, 2097 (1990).
[Crossref]

S. H. Park, R. A. Morgan, Y. Z. Hu, M. Lindberg, S. W. Koch, and N. Peyghambarian, J. Opt. Soc. Am. B 7, 2097 (1990).
[Crossref]

A. Uhrig, L. Banyai, Y. Z. Hu, S. W. Koch, C. Klingshirn, and N. Neuroth, Z. Phys. B 81, 385 (1990).
[Crossref]

Kolenda, J.

U. Woggon, I. Rückmann, J. Kornack, M. Müller, J. Cesnulevicius, M. Petrauskas, and J. Kolenda, J. Cryst. Growth 117, 608 (1992).
[Crossref]

Kornack, J.

U. Woggon, I. Rückmann, J. Kornack, M. Müller, J. Cesnulevicius, M. Petrauskas, and J. Kolenda, J. Cryst. Growth 117, 608 (1992).
[Crossref]

Kottan, A. R.

A. R. Kottan, R. Hull, R. L. Opila, M. G. Bawendi, M. L. Steigerwald, P. J. Caroll, and L. E. Brus, J. Am. Chem. Soc. 112, 1327 (1990).
[Crossref]

Kudryavtsev, I. A.

Lacis, I.

A. Uhrig, A. Wörner, C. Klingshirn, L. Banyai, S. Gaponenko, I. Lacis, N. Neuroth, B. Speith, and K. Remitz, J. Cryst. Growth 117, 598 (1992).
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L. G. Zimin, S. V. Gaponenko, and V. Yu. Lebed, Phys. Status Solidi B 150, 653 (1988).
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M. P. A. Müller, U. Lembke, U. Woggon, and I. Rückmann, J. Non-Cryst. Solids 144, 240 (1992).
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U. Woggon, M. Müller, U. Lembke, I. Rückmann, and J. Cesnulevicius, Superlattices Microstruct. 9, 245 (1991).
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A. P. Alivisatos, A. L. Harris, N. J. Levinos, M. L. Steigerwald, and L. E. Brus, J. Chem. Phys. 89, 4001 (1988).
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I. M. Lifshiz and V. V. Slesov, Zh. Eksp. Teor. Fiz. 35, 479 (1958).

Lindberg, M.

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V. Esch, K. Kang, B. Fluegel, Y. Z. Hu, G. Khitrova, L. C. Liu, and L. C. Risbud, J. Nonlin. Opt. Phys. 1, 25 (1992).
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J. Malhotra, D. J. Hagan, and B. G. Potter, J. Opt. Soc. Am. B 7, 1531 (1991).
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S. Schmitt-Rink, D. A. B. Miller, and D. S. Chemla, Phys. Rev. B 35, 8113 (1987).
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Morgan, R. A.

Müller, M.

U. Woggon, I. Rückmann, J. Kornack, M. Müller, J. Cesnulevicius, M. Petrauskas, and J. Kolenda, J. Cryst. Growth 117, 608 (1992).
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U. Woggon, M. Müller, U. Lembke, I. Rückmann, and J. Cesnulevicius, Superlattices Microstruct. 9, 245 (1991).
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M. P. A. Müller, U. Lembke, U. Woggon, and I. Rückmann, J. Non-Cryst. Solids 144, 240 (1992).
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T. Yanagawa, H. Nakano, and Y. Sasaki, Appl. Phys. Lett. 59, 1690 (1991).
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A. Uhrig, A. Wörner, C. Klingshirn, L. Banyai, S. Gaponenko, I. Lacis, N. Neuroth, B. Speith, and K. Remitz, J. Cryst. Growth 117, 598 (1992).
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A. Uhrig, L. Banyai, Y. Z. Hu, S. W. Koch, C. Klingshirn, and N. Neuroth, Z. Phys. B 81, 385 (1990).
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S. Nomura and T. Kobayashi, Phys. Rev. B 45, 1305 (1992).
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A. R. Kottan, R. Hull, R. L. Opila, M. G. Bawendi, M. L. Steigerwald, P. J. Caroll, and L. E. Brus, J. Am. Chem. Soc. 112, 1327 (1990).
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F. Yan and J. M. Parker, J. Non-Cryst. Solids 112, 277 (1989).
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U. Woggon, I. Rückmann, J. Kornack, M. Müller, J. Cesnulevicius, M. Petrauskas, and J. Kolenda, J. Cryst. Growth 117, 608 (1992).
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J. Malhotra, D. J. Hagan, and B. G. Potter, J. Opt. Soc. Am. B 7, 1531 (1991).
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Ch. Spiegelberg, F. Henneberger, and J. Puls, Superlattices Microstruct. 9, 487 (1991).
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A. Uhrig, A. Wörner, C. Klingshirn, L. Banyai, S. Gaponenko, I. Lacis, N. Neuroth, B. Speith, and K. Remitz, J. Cryst. Growth 117, 598 (1992).
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B. van Wonterghem, S. M. Saltiel, T. E. Dutton, and P. M. Rentzepis, J. Appl. Phys. 66, 4935 (1989).
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V. Esch, K. Kang, B. Fluegel, Y. Z. Hu, G. Khitrova, L. C. Liu, and L. C. Risbud, J. Nonlin. Opt. Phys. 1, 25 (1992).
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L. C. Liu and S. H. Risbud, J. Appl. Phys. 68, 28 (1990).
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P. Roussignol, D. Ricard, C. Flytzanis, and N. Neuroth, Phys. Rev. Lett. 62, 312 (1989).
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P. Roussignol, D. Ricard, J. Lukasik, and C. Flytzanis, J. Opt. Soc. Am. B 4, 5 (1987).
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U. Woggon, I. Rückmann, J. Kornack, M. Müller, J. Cesnulevicius, M. Petrauskas, and J. Kolenda, J. Cryst. Growth 117, 608 (1992).
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M. P. A. Müller, U. Lembke, U. Woggon, and I. Rückmann, J. Non-Cryst. Solids 144, 240 (1992).
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U. Woggon, M. Müller, U. Lembke, I. Rückmann, and J. Cesnulevicius, Superlattices Microstruct. 9, 245 (1991).
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B. van Wonterghem, S. M. Saltiel, T. E. Dutton, and P. M. Rentzepis, J. Appl. Phys. 66, 4935 (1989).
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T. Yanagawa, H. Nakano, and Y. Sasaki, Appl. Phys. Lett. 59, 1690 (1991).
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S. Schmitt-Rink, D. A. B. Miller, and D. S. Chemla, Phys. Rev. B 35, 8113 (1987).
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Simmons, J. H.

B. G. Potter and J. H. Simmons, Phys. Rev. B 37, 10838 (1988).
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I. M. Lifshiz and V. V. Slesov, Zh. Eksp. Teor. Fiz. 35, 479 (1958).

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N. F. Borelli, D. W. Hall, H. J. Holland, and D. W. Smith, J. Appl. Phys. 61, 5399 (1987).
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A. Uhrig, A. Wörner, C. Klingshirn, L. Banyai, S. Gaponenko, I. Lacis, N. Neuroth, B. Speith, and K. Remitz, J. Cryst. Growth 117, 598 (1992).
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Ch. Spiegelberg, F. Henneberger, and J. Puls, Superlattices Microstruct. 9, 487 (1991).
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A. R. Kottan, R. Hull, R. L. Opila, M. G. Bawendi, M. L. Steigerwald, P. J. Caroll, and L. E. Brus, J. Am. Chem. Soc. 112, 1327 (1990).
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M. L. Steigerwald and L. E. Brus, Annu. Rev. Mater. Sci. 19, 471 (1989).
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A. P. Alivisatos, A. L. Harris, N. J. Levinos, M. L. Steigerwald, and L. E. Brus, J. Chem. Phys. 89, 4001 (1988).
[Crossref]

Suna, A.

Tomita, M.

Uhrig, A.

A. Uhrig, A. Wörner, C. Klingshirn, L. Banyai, S. Gaponenko, I. Lacis, N. Neuroth, B. Speith, and K. Remitz, J. Cryst. Growth 117, 598 (1992).
[Crossref]

A. Uhrig, L. Banyai, S. Gaponenko, A. Wörner, N. Neuroth, and C. Klingshirn, Z. Phys. D 20, 345 (1991).
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A. Uhrig, L. Banyai, Y. Z. Hu, S. W. Koch, C. Klingshirn, and N. Neuroth, Z. Phys. B 81, 385 (1990).
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B. van Wonterghem, S. M. Saltiel, T. E. Dutton, and P. M. Rentzepis, J. Appl. Phys. 66, 4935 (1989).
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M. G. Bawendi, P. J. Caroll, W. L. Wilson, and L. E. Brus, J. Chem. Phys. 96, 946 (1992).
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M. P. A. Müller, U. Lembke, U. Woggon, and I. Rückmann, J. Non-Cryst. Solids 144, 240 (1992).
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U. Woggon, I. Rückmann, J. Kornack, M. Müller, J. Cesnulevicius, M. Petrauskas, and J. Kolenda, J. Cryst. Growth 117, 608 (1992).
[Crossref]

U. Woggon, M. Müller, U. Lembke, I. Rückmann, and J. Cesnulevicius, Superlattices Microstruct. 9, 245 (1991).
[Crossref]

Wörner, A.

A. Uhrig, A. Wörner, C. Klingshirn, L. Banyai, S. Gaponenko, I. Lacis, N. Neuroth, B. Speith, and K. Remitz, J. Cryst. Growth 117, 598 (1992).
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A. Uhrig, L. Banyai, S. Gaponenko, A. Wörner, N. Neuroth, and C. Klingshirn, Z. Phys. D 20, 345 (1991).
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Xia, Jian-Bai

Jian-Bai Xia, Phys. Rev. B 40, 8500 (1989).
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Yan, F.

F. Yan and J. M. Parker, J. Non-Cryst. Solids 112, 277 (1989).
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T. Yanagawa, H. Nakano, and Y. Sasaki, Appl. Phys. Lett. 59, 1690 (1991).
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Yazeva, T. V.

Zimin, L. G.

L. G. Zimin, S. V. Gaponenko, and V. Yu. Lebed, Phys. Status Solidi B 150, 653 (1988).
[Crossref]

Annu. Rev. Mater. Sci. (1)

M. L. Steigerwald and L. E. Brus, Annu. Rev. Mater. Sci. 19, 471 (1989).
[Crossref]

Appl. Phys. A (1)

L. E. Brus, Appl. Phys. A 53, 465 (1991).
[Crossref]

Appl. Phys. Lett. (1)

T. Yanagawa, H. Nakano, and Y. Sasaki, Appl. Phys. Lett. 59, 1690 (1991).
[Crossref]

J. Am. Chem. Soc. (1)

A. R. Kottan, R. Hull, R. L. Opila, M. G. Bawendi, M. L. Steigerwald, P. J. Caroll, and L. E. Brus, J. Am. Chem. Soc. 112, 1327 (1990).
[Crossref]

J. Appl. Phys. (3)

N. F. Borelli, D. W. Hall, H. J. Holland, and D. W. Smith, J. Appl. Phys. 61, 5399 (1987).
[Crossref]

L. C. Liu and S. H. Risbud, J. Appl. Phys. 68, 28 (1990).
[Crossref]

B. van Wonterghem, S. M. Saltiel, T. E. Dutton, and P. M. Rentzepis, J. Appl. Phys. 66, 4935 (1989).
[Crossref]

J. Chem. Phys. (2)

A. P. Alivisatos, A. L. Harris, N. J. Levinos, M. L. Steigerwald, and L. E. Brus, J. Chem. Phys. 89, 4001 (1988).
[Crossref]

M. G. Bawendi, P. J. Caroll, W. L. Wilson, and L. E. Brus, J. Chem. Phys. 96, 946 (1992).
[Crossref]

J. Cryst. Growth (3)

A. Uhrig, A. Wörner, C. Klingshirn, L. Banyai, S. Gaponenko, I. Lacis, N. Neuroth, B. Speith, and K. Remitz, J. Cryst. Growth 117, 598 (1992).
[Crossref]

U. Woggon, I. Rückmann, J. Kornack, M. Müller, J. Cesnulevicius, M. Petrauskas, and J. Kolenda, J. Cryst. Growth 117, 608 (1992).
[Crossref]

S. W. Koch, Y. Z. Hu, B. Fluegel, and N. Peyghambarian, J. Cryst. Growth 117, 592 (1992).
[Crossref]

J. Non-Cryst. Solids (2)

F. Yan and J. M. Parker, J. Non-Cryst. Solids 112, 277 (1989).
[Crossref]

M. P. A. Müller, U. Lembke, U. Woggon, and I. Rückmann, J. Non-Cryst. Solids 144, 240 (1992).
[Crossref]

J. Nonlin. Opt. Phys. (1)

V. Esch, K. Kang, B. Fluegel, Y. Z. Hu, G. Khitrova, L. C. Liu, and L. C. Risbud, J. Nonlin. Opt. Phys. 1, 25 (1992).
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Phys. Rev. B (6)

Y. Z. Hu, M. Lindberg, and S. W. Koch, Phys. Rev. B 42, 1713 (1990).
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Jian-Bai Xia, Phys. Rev. B 40, 8500 (1989).
[Crossref]

S. Schmitt-Rink, D. A. B. Miller, and D. S. Chemla, Phys. Rev. B 35, 8113 (1987).
[Crossref]

B. G. Potter and J. H. Simmons, Phys. Rev. B 37, 10838 (1988).
[Crossref]

L. Banyai, P. Gilliot, Y. Z. Hu, and S. W. Koch, Phys. Rev. B 45, 14136 (1992).
[Crossref]

S. Nomura and T. Kobayashi, Phys. Rev. B 45, 1305 (1992).
[Crossref]

Phys. Rev. Lett. (1)

P. Roussignol, D. Ricard, C. Flytzanis, and N. Neuroth, Phys. Rev. Lett. 62, 312 (1989).
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Phys. Scr. (1)

A. I. Ekimov, Phys. Scr. T39, 217 (1991).
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Phys. Status Solidi B (1)

L. G. Zimin, S. V. Gaponenko, and V. Yu. Lebed, Phys. Status Solidi B 150, 653 (1988).
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G. B. Grygoryan, E. M. Kazaryan, Al. L. Efros, and T. V. Yazeva, Sov. Phys. Solid State 32, 1031 (1990).

Superlattices Microstruct. (3)

Ch. Spiegelberg, F. Henneberger, and J. Puls, Superlattices Microstruct. 9, 487 (1991).
[Crossref]

U. Woggon, M. Müller, U. Lembke, I. Rückmann, and J. Cesnulevicius, Superlattices Microstruct. 9, 245 (1991).
[Crossref]

Al. L. Efros, Superlattices Microstruct. 11, 167 (1992).
[Crossref]

Z. Phys. B (1)

A. Uhrig, L. Banyai, Y. Z. Hu, S. W. Koch, C. Klingshirn, and N. Neuroth, Z. Phys. B 81, 385 (1990).
[Crossref]

Z. Phys. D (1)

A. Uhrig, L. Banyai, S. Gaponenko, A. Wörner, N. Neuroth, and C. Klingshirn, Z. Phys. D 20, 345 (1991).
[Crossref]

Zh. Eksp. Teor. Fiz. (1)

I. M. Lifshiz and V. V. Slesov, Zh. Eksp. Teor. Fiz. 35, 479 (1958).

Other (1)

H. Haug and L. Banyai, eds., Optical Switching in Low-Dimensional Systems (Academic, New York, 1989).
[Crossref]

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Figures (8)

Fig. 1
Fig. 1

Linear absorption spectra of some representative samples. (For the parameters of growth see Table 1.) The inset shows the change in absorption for ΔT = ±1 °C at the heat treatment temperature T0 = 590 °C.

Fig. 2
Fig. 2

Influence of an additional nucleation step. Before the coalescence process was carried out at 650 °C for 6 days for samples a and b, an additional low-temperature treatment was performed for sample b at 560 °C for 12 days. The insert shows for comparison the absorption spetra with and without nucleation for growth temperatures going beyond 650 °C: sample 1, 680 °C, 6 days without nucleation; sample 2, 680 °C, 6 days, and low-temperature treatment at 560 °C, 12 days.

Fig. 3
Fig. 3

Linear and differential absorption spectra of CdSxSe1−x QD’s of R = 3.6 nm measured at T = 20 K and an excitation intensity of 100 kW/cm2. The pump energy is indicated by vertical arrows

Fig. 4
Fig. 4

(a) Linear and differential absorption spectra of CdSe QD’s of R = 2.0 nm measured at T = 50 K and an excitation intensity of 100 kW/cm2. The pump energy is indicated by vertical arrows. (b) The same as in (a) but after strong laser illumination with pulses of an intensity of 10 MW/cm2 and a repetition rate of 20 Hz for ~10 min.

Fig. 5
Fig. 5

Narrow-line hole-burning spectrum after laser exposure of the R = 2.0 nm CdSe sample at T = 20 K, an excitation energy of 2.34 eV, and for a low excitation intensity of 30 kW/cm2.

Fig. 6
Fig. 6

(a) Linear and differential absorption spectra of CdSxSe1−x QD’s of R = 2.3 nm measured at T = 20 K and an excitation intensity of 100 kW/cm2. The pump energy is indicated by vertical arrows. For comparison the absorption spectra, 1, without the pump and, 2, with the pump at ħωexc = 2.5 eV (2) are shown. (b) The same as in (a) but after strong laser illumination with pulses of an intensity of 10 MW/cm2 and a repetition rate of 20 Hz for ~10 min.

Fig. 7
Fig. 7

Change in optical density of CdSxSe1−x QD’s of R = 2.3 nm measured at T = 20 K, an excitation intensity of 100 kW/cm2, and for a pump energy of 2.48 eV, 1, before and, 2, after strong laser exposure. Curve 3 shows the combined difference of both contributions.

Fig. 8
Fig. 8

Hole-burning spectra of the R = 2.0 nm CdSe sample at an excitation intensity of 100 kW/cm2, 1, before and, 2, after strong laser exposure. Spectrum 3 is recorded 20 min after spectrum 2 with no further changes at the same spot.

Tables (1)

Tables Icon

Table 1 Parameters of the Heat Treatment Regime of the CdSxSe1−x Samplesa

Equations (3)

Equations on this page are rendered with MathJax. Learn more.

E 1 = E g 0 + C Δ E c ,
R ¯ = α D 0 exp ( Δ E a k T ) t 1 / 3 ,
N = A exp ( Δ E A k T ) exp ( 4 π σ R 0 2 3 k T ) ,

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