Abstract

Fluorescence spectra of acetic acid-water solution excited by ultraviolet (UV) light are studied, and the relationship between fluorescence spectra and molecular association of acetic acid is discussed. The results indicate that when the exciting light wavelength is longer than 246 nm, there are two fluorescence peaks located at 305 and 334 nm, respectively. By measuring the excitation spectra, the optimal wavelengths of the two fluorescence peaks are obtained, which are 258 and 284 nm, respectively. Fluorescence spectra of acetic acid-water solution change with concentrations, which is primarily attributed to changes of molecular association of acetic acid in aqueous solution. Through theoretical analysis, three variations of molecular association have been obtained in acetic acid-water solution, which are the hydrated monomers, the linear dimers, and the water separated dimers. This research can provide references to studies of molecular association of acetic acid-water, especially studies of hydrogen bonds.

© 2009 Chinese Optics Letters

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  1. T. Grossetête, A. Rivaton, J. L. Gardette, C. E. Hoyle, M. Ziemer, D. R. Fagerburg, and H. Clauberg, Polymer 41, 3541 (2000).
  2. T. Suzuki, U. Okuyama, and T. Ichimura, J. Phys. Chem. A 101, 7047 (1997).
  3. N. Moise, C. Carp, and M. L. Pascu, Proc. SPIE 2461, 386 (1995).
  4. G. Verdasco, M. A. Martín, B. del Castillo, P. López-Alvarado, and J. C. Menéndez, Anal. Chim. Acta 303, 73 (1995).
  5. A. R. Zelenchuk, E. Oliva, H. Kaufman, K. T. Schomacker, B. Bandarchi-Chamkhaleh, and J. Pitts, Proc. SPIE 4613, 51 (2002).
  6. J. Semmler and D. E. Irish, J. Solut. Chem. 17, 805 (1988).
  7. J. B. Ng and H. F. Shurvell, J. Phys. Chem. 91, 496 (1987).
  8. N. Tanaka, H. Kitano, and N. Ise, Macromolecules 24, 3017 (1991).
  9. Y. Akiyama, A. Wakisaka, F. Mizukami, and K. Sakaguchi, J. Chem. Soc. 2, 95 (1998).
  10. J. Chocholousová, J. Vacek, and P. Hobza, J. Phys. Chem. A 107, 3086 (2003).
  11. Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Applied Laser (in Chinese) 22, 559 (2002).
  12. Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Laser Technology (in Chinese) 27, 538 (2003).
  13. X. Hu, R. Su, C. Zhang, and X. Wang, Chinese J. Lasers (in Chinese) 35, 115 (2008).
  14. R. Chen, H. Zeng, B. Huang, Z. Huang, and S. Xie, Acta Opt. Sin. (in Chinese) 27, 124 (2007).
  15. J. B. Ng, B. Petelenz, and H. F. Shurvell, Can. J. Chem. 66, 1912 (1988).
  16. N. Nishi, T. Nakabayashi, and K. Kosugi, J. Phys. Chem. A 103, 10851 (1999).
  17. A. J. A. Aquino, D. Tunega, G. Haberhauer, M. H. Gerzabek, and H. Lischka, J. Phys. Chem. A 106, 1862 (2002).
  18. K. Yamamoto and N. Nishi, J. Am. Chem. Soc. 112, 549 (1990).
  19. T. Nakabayashi and N. Nishi, J. Phys. Chem. A 106, 3491 (2002).
  20. E. Ince, J. Chem. Therm. 38, 1669 (2006).
  21. M. Sharma and S. M. Ray, Bioorg. Med. Chem. Lett. 17, 6790 (2007).

2008 (1)

X. Hu, R. Su, C. Zhang, and X. Wang, Chinese J. Lasers (in Chinese) 35, 115 (2008).

2007 (2)

R. Chen, H. Zeng, B. Huang, Z. Huang, and S. Xie, Acta Opt. Sin. (in Chinese) 27, 124 (2007).

M. Sharma and S. M. Ray, Bioorg. Med. Chem. Lett. 17, 6790 (2007).

2006 (1)

E. Ince, J. Chem. Therm. 38, 1669 (2006).

2003 (2)

J. Chocholousová, J. Vacek, and P. Hobza, J. Phys. Chem. A 107, 3086 (2003).

Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Laser Technology (in Chinese) 27, 538 (2003).

2002 (4)

A. J. A. Aquino, D. Tunega, G. Haberhauer, M. H. Gerzabek, and H. Lischka, J. Phys. Chem. A 106, 1862 (2002).

Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Applied Laser (in Chinese) 22, 559 (2002).

A. R. Zelenchuk, E. Oliva, H. Kaufman, K. T. Schomacker, B. Bandarchi-Chamkhaleh, and J. Pitts, Proc. SPIE 4613, 51 (2002).

T. Nakabayashi and N. Nishi, J. Phys. Chem. A 106, 3491 (2002).

2000 (1)

T. Grossetête, A. Rivaton, J. L. Gardette, C. E. Hoyle, M. Ziemer, D. R. Fagerburg, and H. Clauberg, Polymer 41, 3541 (2000).

1999 (1)

N. Nishi, T. Nakabayashi, and K. Kosugi, J. Phys. Chem. A 103, 10851 (1999).

1998 (1)

Y. Akiyama, A. Wakisaka, F. Mizukami, and K. Sakaguchi, J. Chem. Soc. 2, 95 (1998).

1997 (1)

T. Suzuki, U. Okuyama, and T. Ichimura, J. Phys. Chem. A 101, 7047 (1997).

1995 (2)

N. Moise, C. Carp, and M. L. Pascu, Proc. SPIE 2461, 386 (1995).

G. Verdasco, M. A. Martín, B. del Castillo, P. López-Alvarado, and J. C. Menéndez, Anal. Chim. Acta 303, 73 (1995).

1991 (1)

N. Tanaka, H. Kitano, and N. Ise, Macromolecules 24, 3017 (1991).

1990 (1)

K. Yamamoto and N. Nishi, J. Am. Chem. Soc. 112, 549 (1990).

1988 (2)

J. B. Ng, B. Petelenz, and H. F. Shurvell, Can. J. Chem. 66, 1912 (1988).

J. Semmler and D. E. Irish, J. Solut. Chem. 17, 805 (1988).

1987 (1)

J. B. Ng and H. F. Shurvell, J. Phys. Chem. 91, 496 (1987).

Akiyama, Y.

Y. Akiyama, A. Wakisaka, F. Mizukami, and K. Sakaguchi, J. Chem. Soc. 2, 95 (1998).

Aquino, A. J. A.

A. J. A. Aquino, D. Tunega, G. Haberhauer, M. H. Gerzabek, and H. Lischka, J. Phys. Chem. A 106, 1862 (2002).

Bandarchi-Chamkhaleh, B.

A. R. Zelenchuk, E. Oliva, H. Kaufman, K. T. Schomacker, B. Bandarchi-Chamkhaleh, and J. Pitts, Proc. SPIE 4613, 51 (2002).

Carp, C.

N. Moise, C. Carp, and M. L. Pascu, Proc. SPIE 2461, 386 (1995).

Castillo, B. del

G. Verdasco, M. A. Martín, B. del Castillo, P. López-Alvarado, and J. C. Menéndez, Anal. Chim. Acta 303, 73 (1995).

Chen, R.

R. Chen, H. Zeng, B. Huang, Z. Huang, and S. Xie, Acta Opt. Sin. (in Chinese) 27, 124 (2007).

Chocholousová, J.

J. Chocholousová, J. Vacek, and P. Hobza, J. Phys. Chem. A 107, 3086 (2003).

Clauberg, H.

T. Grossetête, A. Rivaton, J. L. Gardette, C. E. Hoyle, M. Ziemer, D. R. Fagerburg, and H. Clauberg, Polymer 41, 3541 (2000).

Fagerburg, D. R.

T. Grossetête, A. Rivaton, J. L. Gardette, C. E. Hoyle, M. Ziemer, D. R. Fagerburg, and H. Clauberg, Polymer 41, 3541 (2000).

Gao, S.

Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Laser Technology (in Chinese) 27, 538 (2003).

Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Applied Laser (in Chinese) 22, 559 (2002).

Gardette, J. L.

T. Grossetête, A. Rivaton, J. L. Gardette, C. E. Hoyle, M. Ziemer, D. R. Fagerburg, and H. Clauberg, Polymer 41, 3541 (2000).

Gerzabek, M. H.

A. J. A. Aquino, D. Tunega, G. Haberhauer, M. H. Gerzabek, and H. Lischka, J. Phys. Chem. A 106, 1862 (2002).

Grossetête, T.

T. Grossetête, A. Rivaton, J. L. Gardette, C. E. Hoyle, M. Ziemer, D. R. Fagerburg, and H. Clauberg, Polymer 41, 3541 (2000).

Haberhauer, G.

A. J. A. Aquino, D. Tunega, G. Haberhauer, M. H. Gerzabek, and H. Lischka, J. Phys. Chem. A 106, 1862 (2002).

Hobza, P.

J. Chocholousová, J. Vacek, and P. Hobza, J. Phys. Chem. A 107, 3086 (2003).

Hoyle, C. E.

T. Grossetête, A. Rivaton, J. L. Gardette, C. E. Hoyle, M. Ziemer, D. R. Fagerburg, and H. Clauberg, Polymer 41, 3541 (2000).

Hu, X.

X. Hu, R. Su, C. Zhang, and X. Wang, Chinese J. Lasers (in Chinese) 35, 115 (2008).

Huang, B.

R. Chen, H. Zeng, B. Huang, Z. Huang, and S. Xie, Acta Opt. Sin. (in Chinese) 27, 124 (2007).

Huang, Z.

R. Chen, H. Zeng, B. Huang, Z. Huang, and S. Xie, Acta Opt. Sin. (in Chinese) 27, 124 (2007).

Ichimura, T.

T. Suzuki, U. Okuyama, and T. Ichimura, J. Phys. Chem. A 101, 7047 (1997).

Ince, E.

E. Ince, J. Chem. Therm. 38, 1669 (2006).

Irish, D. E.

J. Semmler and D. E. Irish, J. Solut. Chem. 17, 805 (1988).

Ise, N.

N. Tanaka, H. Kitano, and N. Ise, Macromolecules 24, 3017 (1991).

Kaufman, H.

A. R. Zelenchuk, E. Oliva, H. Kaufman, K. T. Schomacker, B. Bandarchi-Chamkhaleh, and J. Pitts, Proc. SPIE 4613, 51 (2002).

Kitano, H.

N. Tanaka, H. Kitano, and N. Ise, Macromolecules 24, 3017 (1991).

Kosugi, K.

N. Nishi, T. Nakabayashi, and K. Kosugi, J. Phys. Chem. A 103, 10851 (1999).

Lan, X.

Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Laser Technology (in Chinese) 27, 538 (2003).

Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Applied Laser (in Chinese) 22, 559 (2002).

Lischka, H.

A. J. A. Aquino, D. Tunega, G. Haberhauer, M. H. Gerzabek, and H. Lischka, J. Phys. Chem. A 106, 1862 (2002).

Liu, Y.

Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Laser Technology (in Chinese) 27, 538 (2003).

Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Applied Laser (in Chinese) 22, 559 (2002).

López-Alvarado, P.

G. Verdasco, M. A. Martín, B. del Castillo, P. López-Alvarado, and J. C. Menéndez, Anal. Chim. Acta 303, 73 (1995).

Lu, J.

Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Laser Technology (in Chinese) 27, 538 (2003).

Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Applied Laser (in Chinese) 22, 559 (2002).

Martín, M. A.

G. Verdasco, M. A. Martín, B. del Castillo, P. López-Alvarado, and J. C. Menéndez, Anal. Chim. Acta 303, 73 (1995).

Menéndez, J. C.

G. Verdasco, M. A. Martín, B. del Castillo, P. López-Alvarado, and J. C. Menéndez, Anal. Chim. Acta 303, 73 (1995).

Mizukami, F.

Y. Akiyama, A. Wakisaka, F. Mizukami, and K. Sakaguchi, J. Chem. Soc. 2, 95 (1998).

Moise, N.

N. Moise, C. Carp, and M. L. Pascu, Proc. SPIE 2461, 386 (1995).

Nakabayashi, T.

T. Nakabayashi and N. Nishi, J. Phys. Chem. A 106, 3491 (2002).

N. Nishi, T. Nakabayashi, and K. Kosugi, J. Phys. Chem. A 103, 10851 (1999).

Ng, J. B.

J. B. Ng, B. Petelenz, and H. F. Shurvell, Can. J. Chem. 66, 1912 (1988).

J. B. Ng and H. F. Shurvell, J. Phys. Chem. 91, 496 (1987).

Ni, X.

Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Laser Technology (in Chinese) 27, 538 (2003).

Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Applied Laser (in Chinese) 22, 559 (2002).

Nishi, N.

T. Nakabayashi and N. Nishi, J. Phys. Chem. A 106, 3491 (2002).

N. Nishi, T. Nakabayashi, and K. Kosugi, J. Phys. Chem. A 103, 10851 (1999).

K. Yamamoto and N. Nishi, J. Am. Chem. Soc. 112, 549 (1990).

Okuyama, U.

T. Suzuki, U. Okuyama, and T. Ichimura, J. Phys. Chem. A 101, 7047 (1997).

Oliva, E.

A. R. Zelenchuk, E. Oliva, H. Kaufman, K. T. Schomacker, B. Bandarchi-Chamkhaleh, and J. Pitts, Proc. SPIE 4613, 51 (2002).

Pascu, M. L.

N. Moise, C. Carp, and M. L. Pascu, Proc. SPIE 2461, 386 (1995).

Petelenz, B.

J. B. Ng, B. Petelenz, and H. F. Shurvell, Can. J. Chem. 66, 1912 (1988).

Pitts, J.

A. R. Zelenchuk, E. Oliva, H. Kaufman, K. T. Schomacker, B. Bandarchi-Chamkhaleh, and J. Pitts, Proc. SPIE 4613, 51 (2002).

Ray, S. M.

M. Sharma and S. M. Ray, Bioorg. Med. Chem. Lett. 17, 6790 (2007).

Rivaton, A.

T. Grossetête, A. Rivaton, J. L. Gardette, C. E. Hoyle, M. Ziemer, D. R. Fagerburg, and H. Clauberg, Polymer 41, 3541 (2000).

Sakaguchi, K.

Y. Akiyama, A. Wakisaka, F. Mizukami, and K. Sakaguchi, J. Chem. Soc. 2, 95 (1998).

Schomacker, K. T.

A. R. Zelenchuk, E. Oliva, H. Kaufman, K. T. Schomacker, B. Bandarchi-Chamkhaleh, and J. Pitts, Proc. SPIE 4613, 51 (2002).

Semmler, J.

J. Semmler and D. E. Irish, J. Solut. Chem. 17, 805 (1988).

Sharma, M.

M. Sharma and S. M. Ray, Bioorg. Med. Chem. Lett. 17, 6790 (2007).

Shen, Z.

Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Laser Technology (in Chinese) 27, 538 (2003).

Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Applied Laser (in Chinese) 22, 559 (2002).

Shurvell, H. F.

J. B. Ng, B. Petelenz, and H. F. Shurvell, Can. J. Chem. 66, 1912 (1988).

J. B. Ng and H. F. Shurvell, J. Phys. Chem. 91, 496 (1987).

Su, R.

X. Hu, R. Su, C. Zhang, and X. Wang, Chinese J. Lasers (in Chinese) 35, 115 (2008).

Suzuki, T.

T. Suzuki, U. Okuyama, and T. Ichimura, J. Phys. Chem. A 101, 7047 (1997).

Tanaka, N.

N. Tanaka, H. Kitano, and N. Ise, Macromolecules 24, 3017 (1991).

Tunega, D.

A. J. A. Aquino, D. Tunega, G. Haberhauer, M. H. Gerzabek, and H. Lischka, J. Phys. Chem. A 106, 1862 (2002).

Vacek, J.

J. Chocholousová, J. Vacek, and P. Hobza, J. Phys. Chem. A 107, 3086 (2003).

Verdasco, G.

G. Verdasco, M. A. Martín, B. del Castillo, P. López-Alvarado, and J. C. Menéndez, Anal. Chim. Acta 303, 73 (1995).

Wakisaka, A.

Y. Akiyama, A. Wakisaka, F. Mizukami, and K. Sakaguchi, J. Chem. Soc. 2, 95 (1998).

Wang, X.

X. Hu, R. Su, C. Zhang, and X. Wang, Chinese J. Lasers (in Chinese) 35, 115 (2008).

Xie, S.

R. Chen, H. Zeng, B. Huang, Z. Huang, and S. Xie, Acta Opt. Sin. (in Chinese) 27, 124 (2007).

Yamamoto, K.

K. Yamamoto and N. Nishi, J. Am. Chem. Soc. 112, 549 (1990).

Zelenchuk, A. R.

A. R. Zelenchuk, E. Oliva, H. Kaufman, K. T. Schomacker, B. Bandarchi-Chamkhaleh, and J. Pitts, Proc. SPIE 4613, 51 (2002).

Zeng, H.

R. Chen, H. Zeng, B. Huang, Z. Huang, and S. Xie, Acta Opt. Sin. (in Chinese) 27, 124 (2007).

Zhang, C.

X. Hu, R. Su, C. Zhang, and X. Wang, Chinese J. Lasers (in Chinese) 35, 115 (2008).

Ziemer, M.

T. Grossetête, A. Rivaton, J. L. Gardette, C. E. Hoyle, M. Ziemer, D. R. Fagerburg, and H. Clauberg, Polymer 41, 3541 (2000).

Acta Opt. Sin. (in Chinese) (1)

R. Chen, H. Zeng, B. Huang, Z. Huang, and S. Xie, Acta Opt. Sin. (in Chinese) 27, 124 (2007).

Anal. Chim. Acta (1)

G. Verdasco, M. A. Martín, B. del Castillo, P. López-Alvarado, and J. C. Menéndez, Anal. Chim. Acta 303, 73 (1995).

Applied Laser (in Chinese) (1)

Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Applied Laser (in Chinese) 22, 559 (2002).

Bioorg. Med. Chem. Lett. (1)

M. Sharma and S. M. Ray, Bioorg. Med. Chem. Lett. 17, 6790 (2007).

Can. J. Chem. (1)

J. B. Ng, B. Petelenz, and H. F. Shurvell, Can. J. Chem. 66, 1912 (1988).

Chinese J. Lasers (in Chinese) (1)

X. Hu, R. Su, C. Zhang, and X. Wang, Chinese J. Lasers (in Chinese) 35, 115 (2008).

J. Am. Chem. Soc. (1)

K. Yamamoto and N. Nishi, J. Am. Chem. Soc. 112, 549 (1990).

J. Chem. Soc. (1)

Y. Akiyama, A. Wakisaka, F. Mizukami, and K. Sakaguchi, J. Chem. Soc. 2, 95 (1998).

J. Chem. Therm. (1)

E. Ince, J. Chem. Therm. 38, 1669 (2006).

J. Phys. Chem. (1)

J. B. Ng and H. F. Shurvell, J. Phys. Chem. 91, 496 (1987).

J. Phys. Chem. A (5)

T. Suzuki, U. Okuyama, and T. Ichimura, J. Phys. Chem. A 101, 7047 (1997).

J. Chocholousová, J. Vacek, and P. Hobza, J. Phys. Chem. A 107, 3086 (2003).

N. Nishi, T. Nakabayashi, and K. Kosugi, J. Phys. Chem. A 103, 10851 (1999).

A. J. A. Aquino, D. Tunega, G. Haberhauer, M. H. Gerzabek, and H. Lischka, J. Phys. Chem. A 106, 1862 (2002).

T. Nakabayashi and N. Nishi, J. Phys. Chem. A 106, 3491 (2002).

J. Solut. Chem. (1)

J. Semmler and D. E. Irish, J. Solut. Chem. 17, 805 (1988).

Laser Technology (in Chinese) (1)

Y. Liu, X. Lan, S. Gao, Z. Shen, J. Lu, and X. Ni, Laser Technology (in Chinese) 27, 538 (2003).

Macromolecules (1)

N. Tanaka, H. Kitano, and N. Ise, Macromolecules 24, 3017 (1991).

Polymer (1)

T. Grossetête, A. Rivaton, J. L. Gardette, C. E. Hoyle, M. Ziemer, D. R. Fagerburg, and H. Clauberg, Polymer 41, 3541 (2000).

Proc. SPIE (2)

N. Moise, C. Carp, and M. L. Pascu, Proc. SPIE 2461, 386 (1995).

A. R. Zelenchuk, E. Oliva, H. Kaufman, K. T. Schomacker, B. Bandarchi-Chamkhaleh, and J. Pitts, Proc. SPIE 4613, 51 (2002).

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