Abstract

A series of diarylethene derivatives with two-photon absorption was designed and synthesized. The nonlinear properties of two-photon induced fluorescence of the compounds were examined. A strategy for the design of molecules with large two-photon absorption (TRA) was developed. These compounds were also successfully applied in two-photon three-dimensional (3D) optical data storage based on single beam two-photon femtosecond writing and one-photon fluorescence reading.

© 2005 Chinese Optics Letters

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H. Guo, F. Zhang, G. Wu, F. Sun, and S. Pu, Opt. Mater. 22, 269 (2003).

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M. Irie, Chem. Rev. 100, 1685 (2000).

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A. S. Dvornikov, Y. Liang, I. V. Tomov, and P. M. Rentzepis, Proc. SPIE 3802, 192 (1999).

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D. Day and M. Gu, Appl. Opt. 37, 6299 (1998).

T. Kogej, D. Beljonne, F. Meyers, J. W. Perry, S. R. Marder, and J. L. Bredas, Chem. Phys. Lett. 298, 1 (1998).

M. Albota, D. Beljonne, J.-L. Bredas, J. E. Ehrlich, J.-Y. Fu, A. A. Heikal, S. E. Hess, T. Kogej, M. D. Levin, S. R. Marder, D. Mccord-Maughon, J. W. Perry, H. Rockel, M. Rumi, G. Subramaniam, W. W. Webb, X.-L. Wu, and C. Xu, Science 281, 1653 (1998).

A. Toriumi and S. Kawata, Opt. Lett. 23, 1924 (1998).

1990

Appl. Opt.

Chem. Phys. Lett.

T. Kogej, D. Beljonne, F. Meyers, J. W. Perry, S. R. Marder, and J. L. Bredas, Chem. Phys. Lett. 298, 1 (1998).

Chem. Rev.

M. Irie, Chem. Rev. 100, 1685 (2000).

Opt. Lett.

Opt. Mater.

H. Guo, F. Zhang, G. Wu, F. Sun, and S. Pu, Opt. Mater. 22, 269 (2003).

Proc. SPIE

A. S. Dvornikov, Y. Liang, I. V. Tomov, and P. M. Rentzepis, Proc. SPIE 3802, 192 (1999).

Science

M. Albota, D. Beljonne, J.-L. Bredas, J. E. Ehrlich, J.-Y. Fu, A. A. Heikal, S. E. Hess, T. Kogej, M. D. Levin, S. R. Marder, D. Mccord-Maughon, J. W. Perry, H. Rockel, M. Rumi, G. Subramaniam, W. W. Webb, X.-L. Wu, and C. Xu, Science 281, 1653 (1998).

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