Abstract

This study indicates that intermolecular complexes exist between tetraal-kylurea and carbon tetrachloride and between tetraalkylurea and chloroform. The type of complex or complexes formed is dependent upon the mole % CCl₄/C₆H₁₄ or mole % CHCl₃/C₆H₁₄. Intermolecular hydrogen-bonded complexes between tetraalkylurea and chloroform (such as I; I and II; II and III; and III) are formed as the mole % CHCl₃/C₆H₁₄ increases. The steady decrease in the <i>v</i>C=O frequency is attributed in part to the bulk dielectric effects of the solvent system.

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