Experiments have been performed to investigate the possibility of detecting low concentrations of SO<sub>2</sub> using CARS spectroscopy. The experiments were also aimed at high-temperature investigations both in a heated cell and in a flame. During the cell measurements it was clearly revealed that the temperature has a dramatic influence on the shape of the CARS spectra, indicating a good potential for thermometry using SO<sub>2</sub> and CARS spectroscopy.

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