Raman scattering of actinide (VI) ions from carbonate media were obtained. Results indicate bidentate complexation of carbonate and linear geometry for the AnO<sup>2+</sup><sub>2</sub> ions. The trend of the frequency position of the <i>v</i><sub>1</sub> vibration in AnO<sup>2+</sup><sub>2</sub> ions is U > Np > Pu > Am in both acid and basic solutions, with higher frequencies occurring in acid media.

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