Single graphene derivative layer as a hole transport in organic solar
cells based on PBDB-T:ITIC

Olivia Amargós-Reyes; Irving Caballero-Quintana; José-Luis Maldonado; Juan Nicasio-Collazo; Daniel Romero-Borja

doi:10.1364/AO.402510

Applied Optics
Vol. 59,
Issue 27,
pp. 8285-8292
(2020)
•https://doi.org/10.1364/AO.402510

Single graphene derivative layer as a hole transport in organic solar cells based on PBDB-T:ITIC

Olivia Amargós-Reyes, Irving Caballero-Quintana, José-Luis Maldonado, Juan Nicasio-Collazo, and Daniel Romero-Borja

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Olivia Amargós-Reyes, Irving Caballero-Quintana, José-Luis Maldonado, Juan Nicasio-Collazo, and Daniel Romero-Borja, "Single graphene derivative layer as a hole transport in organic solar cells based on PBDB-T:ITIC," Appl. Opt. 59, 8285-8292 (2020)

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- Optical Devices, Sensors, and Detectors
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About this Article
History
- Original Manuscript: July 10, 2020
- Revised Manuscript: August 19, 2020
- Manuscript Accepted: August 25, 2020
- Published: September 16, 2020

Abstract

A layer of fluorinated reduced graphene oxide (FrGO), as an alternative hole transport (HTL) in organic solar cells (OSCs) based on a PBDB-T:ITIC active layer, is reported. OSC configuration is ITO/HTL/PBDB-T:ITIC/PFN/FM; FM is Field’s metal, a eutectic alloy deposited at room atmosphere. PEDOT:PSS, FrGO/PEDOT:PSS, and FrGO are tested as HTLs; the average efficiencies of 8.8, 8.2, and 5.3%, respectively, are reached. Inhomogeneity of the FrGO layer is determined as the main factor that affects the photovoltaic behavior and stability. Device stability is very acceptable, sometimes with a superior behavior than data previously reported; FM also could potentially contribute to this enhanced stability.

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HTL	$V_{oc}$ $(V)$	$J_{sc}$ $(m A / {c m}^{2})$	FF	PCE (%)	$R_{s}$ $(Ω {c m}^{2})$	$R_{sh}$ $(Ω {c m}^{2})$
PEDOT:PSS	0.88	16.0 (14.3) ^c	0.63	8.9 (8.8)	3	340
FrGO/PEDOT:PSS	0.87	14.7 (13.9) ^c	0.65	8.4 (8.2)	5	250
FrGO	0.72	13.6 (12.5) ^c	0.56	5.4 (5.3)	10	160

HTL	Active layer	$V_{oc}$ $(V)$	$J_{sc}$ $(m A / {c m}^{2})$	FF	PCE (%)	Lifetime ( $d a y s > 50 %$ )	Ref.
GOs/PEDOT:PSS	PBDB-T:ITIC	0.9(0.89)	15.1(15.1)	0.66(0.64)	8.9(8.6)	$> 42$	[16]
G-PEDOT:PSS	$P 3 H T : {P C}_{60} B M$	0.48(0.52)	13.6(13.3)	0.68(0.60)	4.5(4.2)	–	[17]
PEDOT:PSS/GO	$P 3 H T : {P C}_{60} B M$	0.63(0.62)	8.6(7.1)	0.63(0.68)	3.4(3.0)	–	[23]
GO/PEDOT:PSS	$P 3 H T : {P C}_{60} B M$	0.49(0.46)	15.4(13.4)	0.64(0.63)	4.8(4.0)	$\sim 10$	[39]
GO-Cl	$P 3 H T : {P C}_{60} B M$	0.60(0.60)	10.2(8.6)	0.61(0.63)	3.7(3.2)	$\sim 2$	[41]
pr-GO1	$P 3 H T : {P C}_{60} B M$	0.59(0.60)	9.3(9.4)	0.67(0.65)	3.6(3.6)	$\sim 13$	[42]
GO	$P 3 H T : {P C}_{60} B M$	0.60(0.60)	9.6(9.2)	0.51(0.52)	2.9(2.9)	$\sim 2$	[43]
MR-GO	$P 3 H T : {P C}_{60} B M$	0.62(0.62)	8.8(7.4)	0.65(0.64)	3.6(3.0)	$> 42$	[44]
GO	$P 3 H T : {P C}_{60} B M$	0.57(0.58)	11.4(11.2)	0.54(0.57)	3.5(3.6)	–	[45]
GO/ $M o O_{3 - x}$	$P 3 H T : {P C}_{60} B M$	0.63(0.64)	9.1(8.8)	0.71(0.66)	4.1(3.7)	$> 40$	[46]
FrGO	P3HT:ICBA	0.83(0.85)	8.7(9.1)	0.64(0.60)	4.6(4.7)	$> 2$	[47]
FrGO/PEDOT:PSS	$P T B 7 : {P C}_{71} B M$	0.78(0.77)	15.3(15.1)	0.63(0.62)	7.5(7.3)	$> 29$	[30]
FrGO	$P T B 7 : {P C}_{71} B M$	0.68(0.77)	14.8(15.1)	0.57(0.62)	5.7(7.3)	$> 29$	[30]
6-rGO	$P T B 7 : {P C}_{71} B M$	0.70(0.76)	13.4(14.2)	0.58(0.51)	5.5(5.5)	–	[32]
FrGO	$P T B 7 : {P C}_{71} B M$	0.70(0.71)	14.8(15.1)	0.65(0.64)	6.7(6.9)	$> 2$	[47]
VP-rGO	$P T B 7 - T h : {P C}_{71} B M$	0.78(0.77)	15.3(15.9)	0.69(0.68)	8.3(8.3)	–	[18]
FrGO	$P T B 7 - T h : {P C}_{71} B M$	0.79(0.78)	16.9(16.4)	0.65(0.62)	8.6(7.9)	$> 3$	[38]
GMo2/PEDOT:PSS	$P T B 7 - T h : {P C}_{71} B M$	0.77(0.77)	17.2(16.7)	0.72(0.68)	9.4(9.0)	–	[48]
G- $M o O_{3}$	$P C D T B T : {P C}_{71} B M$	0.86(0.86 ^c )	12.8(11.0 ^c )	0.64(0.61 ^c )	7.1(5.7 ^c )	–	[27]
GO-Cl	$P C D T B T : {P C}_{71} B M$	0.88(0.88)	13.7(11.3)	0.55(0.55)	6.6(5.5)	$\sim 2$	[41]
GO/ $M o O_{3 - x}$	$P T h B D T P : {P C}_{71} B M$	0.97(0.98)	12.2(12.0)	0.68(0.67)	8.1(7.9)	–	[46]

HTL	$V_{oc}$ $(V)$	$J_{sc}$ $(m A / {c m}^{2})$	FF	PCE (%)	$R_{s}$ $(Ω {c m}^{2})$	$R_{sh}$ $(Ω {c m}^{2})$
PEDOT:PSS	0.88	16.0 (14.3) ^c	0.63	8.9 (8.8)	3	340
FrGO/PEDOT:PSS	0.87	14.7 (13.9) ^c	0.65	8.4 (8.2)	5	250
FrGO	0.72	13.6 (12.5) ^c	0.56	5.4 (5.3)	10	160

HTL	Active layer	$V_{oc}$ $(V)$	$J_{sc}$ $(m A / {c m}^{2})$	FF	PCE (%)	Lifetime ( $d a y s > 50 %$ )	Ref.
GOs/PEDOT:PSS	PBDB-T:ITIC	0.9(0.89)	15.1(15.1)	0.66(0.64)	8.9(8.6)	$> 42$	[16]
G-PEDOT:PSS	$P 3 H T : {P C}_{60} B M$	0.48(0.52)	13.6(13.3)	0.68(0.60)	4.5(4.2)	–	[17]
PEDOT:PSS/GO	$P 3 H T : {P C}_{60} B M$	0.63(0.62)	8.6(7.1)	0.63(0.68)	3.4(3.0)	–	[23]
GO/PEDOT:PSS	$P 3 H T : {P C}_{60} B M$	0.49(0.46)	15.4(13.4)	0.64(0.63)	4.8(4.0)	$\sim 10$	[39]
GO-Cl	$P 3 H T : {P C}_{60} B M$	0.60(0.60)	10.2(8.6)	0.61(0.63)	3.7(3.2)	$\sim 2$	[41]
pr-GO1	$P 3 H T : {P C}_{60} B M$	0.59(0.60)	9.3(9.4)	0.67(0.65)	3.6(3.6)	$\sim 13$	[42]
GO	$P 3 H T : {P C}_{60} B M$	0.60(0.60)	9.6(9.2)	0.51(0.52)	2.9(2.9)	$\sim 2$	[43]
MR-GO	$P 3 H T : {P C}_{60} B M$	0.62(0.62)	8.8(7.4)	0.65(0.64)	3.6(3.0)	$> 42$	[44]
GO	$P 3 H T : {P C}_{60} B M$	0.57(0.58)	11.4(11.2)	0.54(0.57)	3.5(3.6)	–	[45]
GO/ $M o O_{3 - x}$	$P 3 H T : {P C}_{60} B M$	0.63(0.64)	9.1(8.8)	0.71(0.66)	4.1(3.7)	$> 40$	[46]
FrGO	P3HT:ICBA	0.83(0.85)	8.7(9.1)	0.64(0.60)	4.6(4.7)	$> 2$	[47]
FrGO/PEDOT:PSS	$P T B 7 : {P C}_{71} B M$	0.78(0.77)	15.3(15.1)	0.63(0.62)	7.5(7.3)	$> 29$	[30]
FrGO	$P T B 7 : {P C}_{71} B M$	0.68(0.77)	14.8(15.1)	0.57(0.62)	5.7(7.3)	$> 29$	[30]
6-rGO	$P T B 7 : {P C}_{71} B M$	0.70(0.76)	13.4(14.2)	0.58(0.51)	5.5(5.5)	–	[32]
FrGO	$P T B 7 : {P C}_{71} B M$	0.70(0.71)	14.8(15.1)	0.65(0.64)	6.7(6.9)	$> 2$	[47]
VP-rGO	$P T B 7 - T h : {P C}_{71} B M$	0.78(0.77)	15.3(15.9)	0.69(0.68)	8.3(8.3)	–	[18]
FrGO	$P T B 7 - T h : {P C}_{71} B M$	0.79(0.78)	16.9(16.4)	0.65(0.62)	8.6(7.9)	$> 3$	[38]
GMo2/PEDOT:PSS	$P T B 7 - T h : {P C}_{71} B M$	0.77(0.77)	17.2(16.7)	0.72(0.68)	9.4(9.0)	–	[48]
G- $M o O_{3}$	$P C D T B T : {P C}_{71} B M$	0.86(0.86 ^c )	12.8(11.0 ^c )	0.64(0.61 ^c )	7.1(5.7 ^c )	–	[27]
GO-Cl	$P C D T B T : {P C}_{71} B M$	0.88(0.88)	13.7(11.3)	0.55(0.55)	6.6(5.5)	$\sim 2$	[41]
GO/ $M o O_{3 - x}$	$P T h B D T P : {P C}_{71} B M$	0.97(0.98)	12.2(12.0)	0.68(0.67)	8.1(7.9)	–	[46]

Abstract

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Applied Optics