Abstract

Polarization modulation of two-photon excited fluorescence in a V-shaped dipicolinate-triphenylamine compound was investigated with 100 fs 800 nm laser pulses. The peak fluorescence intensity versus the input irradiance was measured to meet a square dependence, which offered evidence for two-photon excited fluorescence. The variations of the two-photon excited fluorescence intensity showed strong response to the different polarized incident lights and were tightly dependent on the linearly polarized component of the incident light. Furthermore, the polarization modulation efficiency of the two-photon excited fluorescence had an obvious concentration dependence when the concentration of solution was under $2.5\times {10}^{-4}\mathrm{mol}/\mathrm{L}$. The enhancement of modulation efficiency was attributed to the concentration dependence of the two-photon absorption cross section.

© 2015 Optical Society of America

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