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Precise measurement of the rotational Raman gain coefficient in para-hydrogen by the large-signal method

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Abstract

The plane-wave gain coefficient of stimulated rotational Raman scattering in para-H2 was determined for CO2 laser-pumping pulses. Difficulties caused by lowered substantial gain for stimulated scattering in the infrared region were overcome by measuring converted energies instead of powers in the large-signal region. The measured gain coefficients showed excellent agreement with theoretical values.

© 1992 Optical Society of America

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