Abstract

The isotopic selectivity of multiple-photon dissociation (MPD) was first demonstrated on 10BCl3 and 11BCl3 molecules by Ambartsumiam et al. in 1974. This paper discusses experiments with MPD as an isotope enrichment method.

© 1984 Optical Society of America

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  1. R. V. Ambartsumian et al., Pis’ma Zh. Eksp. Teor. Fiz. 20, 597 (1974) [JETP Lett. 20, 273 (1974)].
  2. N. V. Karlov, A. M. Prokhorov, Usp. Fiz. Nauk 118, 583 (1976) [Sov. Phys. Usp. 19, 285 (1976)].
    [CrossRef]
  3. V. S. Letokhov, C. B. Moore, Chemical and Biochemical Applications of Lasers, C. B. Moore, Ed. (Academic, New York, 1977), Vol. 3, p. 1.
  4. V. N. Bagratashvili, V. S. Letokhov, A. A. Makarov, E. A. Ryabov, Multiple-Photon Processes in Molecules under IR Laser Radiation (Viniti, Moscow, 1981).
  5. I. G. Gverdtsiteli, E. D. Oziashvili, Production of Isotopes (Atomizdat, Moscow, 1973).
  6. O. G. Sarishvili et al., At. Energ. 43, 210 (1977).
    [CrossRef]
  7. A. B. Bakhatdze, Stable Isotopes in the Life Sciences (International Atomic Energy Agency, Vienna, 1977).
  8. K. Cohen, The Theory of Isotope Separation (McGraw-Hill, New York, 1951).
  9. G. I. Abdushelishvili et al., Pis’ma Zh. Tekh. Fiz. 5, 14849 (1979) [Sov. Tech. Phys. Lett. 5, 350 (1979)].
  10. G. I. Abdushelishvili et al., Kvantovaya Elektron. (Moscow) 8, 534 (1981) [Sov. J. Quantum Electron. 12, 459 (1982)].
  11. G. I. Abdushelishvili et al., in Proceedings, Fourth International Symposium on Gas Flow and Chemical Lasers, Stresa, 1982.
  12. V. Yu. Baranov et al., Kvantovaya Elektron. (Moscow) 6, 811 (1979) [Sov. J. Quantum. Electron. 9, 480 (1979)].
  13. M. Gauthier, W. S. Nip, P. A. Hackett, C. Willis, Chem. Phys. Lett. 69, 372 (1980).
    [CrossRef]
  14. V. S. Doljikov, V. R. Kolomisky, E. A. Ryabov, Chem. Phys. Lett. 80, 472 (1981).
    [CrossRef]
  15. O. N. Avatokov et al., in Proceedings, Eleventh Conference on Coherent and Nonlinear Optics, Erevan, 1982, p. 672.

1981

G. I. Abdushelishvili et al., Kvantovaya Elektron. (Moscow) 8, 534 (1981) [Sov. J. Quantum Electron. 12, 459 (1982)].

V. S. Doljikov, V. R. Kolomisky, E. A. Ryabov, Chem. Phys. Lett. 80, 472 (1981).
[CrossRef]

1980

M. Gauthier, W. S. Nip, P. A. Hackett, C. Willis, Chem. Phys. Lett. 69, 372 (1980).
[CrossRef]

1979

V. Yu. Baranov et al., Kvantovaya Elektron. (Moscow) 6, 811 (1979) [Sov. J. Quantum. Electron. 9, 480 (1979)].

G. I. Abdushelishvili et al., Pis’ma Zh. Tekh. Fiz. 5, 14849 (1979) [Sov. Tech. Phys. Lett. 5, 350 (1979)].

1977

O. G. Sarishvili et al., At. Energ. 43, 210 (1977).
[CrossRef]

1976

N. V. Karlov, A. M. Prokhorov, Usp. Fiz. Nauk 118, 583 (1976) [Sov. Phys. Usp. 19, 285 (1976)].
[CrossRef]

1974

R. V. Ambartsumian et al., Pis’ma Zh. Eksp. Teor. Fiz. 20, 597 (1974) [JETP Lett. 20, 273 (1974)].

Abdushelishvili, G. I.

G. I. Abdushelishvili et al., Kvantovaya Elektron. (Moscow) 8, 534 (1981) [Sov. J. Quantum Electron. 12, 459 (1982)].

G. I. Abdushelishvili et al., Pis’ma Zh. Tekh. Fiz. 5, 14849 (1979) [Sov. Tech. Phys. Lett. 5, 350 (1979)].

G. I. Abdushelishvili et al., in Proceedings, Fourth International Symposium on Gas Flow and Chemical Lasers, Stresa, 1982.

Ambartsumian, R. V.

R. V. Ambartsumian et al., Pis’ma Zh. Eksp. Teor. Fiz. 20, 597 (1974) [JETP Lett. 20, 273 (1974)].

Avatokov, O. N.

O. N. Avatokov et al., in Proceedings, Eleventh Conference on Coherent and Nonlinear Optics, Erevan, 1982, p. 672.

Bagratashvili, V. N.

V. N. Bagratashvili, V. S. Letokhov, A. A. Makarov, E. A. Ryabov, Multiple-Photon Processes in Molecules under IR Laser Radiation (Viniti, Moscow, 1981).

Bakhatdze, A. B.

A. B. Bakhatdze, Stable Isotopes in the Life Sciences (International Atomic Energy Agency, Vienna, 1977).

Baranov, V. Yu.

V. Yu. Baranov et al., Kvantovaya Elektron. (Moscow) 6, 811 (1979) [Sov. J. Quantum. Electron. 9, 480 (1979)].

Cohen, K.

K. Cohen, The Theory of Isotope Separation (McGraw-Hill, New York, 1951).

Doljikov, V. S.

V. S. Doljikov, V. R. Kolomisky, E. A. Ryabov, Chem. Phys. Lett. 80, 472 (1981).
[CrossRef]

Gauthier, M.

M. Gauthier, W. S. Nip, P. A. Hackett, C. Willis, Chem. Phys. Lett. 69, 372 (1980).
[CrossRef]

Gverdtsiteli, I. G.

I. G. Gverdtsiteli, E. D. Oziashvili, Production of Isotopes (Atomizdat, Moscow, 1973).

Hackett, P. A.

M. Gauthier, W. S. Nip, P. A. Hackett, C. Willis, Chem. Phys. Lett. 69, 372 (1980).
[CrossRef]

Karlov, N. V.

N. V. Karlov, A. M. Prokhorov, Usp. Fiz. Nauk 118, 583 (1976) [Sov. Phys. Usp. 19, 285 (1976)].
[CrossRef]

Kolomisky, V. R.

V. S. Doljikov, V. R. Kolomisky, E. A. Ryabov, Chem. Phys. Lett. 80, 472 (1981).
[CrossRef]

Letokhov, V. S.

V. S. Letokhov, C. B. Moore, Chemical and Biochemical Applications of Lasers, C. B. Moore, Ed. (Academic, New York, 1977), Vol. 3, p. 1.

V. N. Bagratashvili, V. S. Letokhov, A. A. Makarov, E. A. Ryabov, Multiple-Photon Processes in Molecules under IR Laser Radiation (Viniti, Moscow, 1981).

Makarov, A. A.

V. N. Bagratashvili, V. S. Letokhov, A. A. Makarov, E. A. Ryabov, Multiple-Photon Processes in Molecules under IR Laser Radiation (Viniti, Moscow, 1981).

Moore, C. B.

V. S. Letokhov, C. B. Moore, Chemical and Biochemical Applications of Lasers, C. B. Moore, Ed. (Academic, New York, 1977), Vol. 3, p. 1.

Nip, W. S.

M. Gauthier, W. S. Nip, P. A. Hackett, C. Willis, Chem. Phys. Lett. 69, 372 (1980).
[CrossRef]

Oziashvili, E. D.

I. G. Gverdtsiteli, E. D. Oziashvili, Production of Isotopes (Atomizdat, Moscow, 1973).

Prokhorov, A. M.

N. V. Karlov, A. M. Prokhorov, Usp. Fiz. Nauk 118, 583 (1976) [Sov. Phys. Usp. 19, 285 (1976)].
[CrossRef]

Ryabov, E. A.

V. S. Doljikov, V. R. Kolomisky, E. A. Ryabov, Chem. Phys. Lett. 80, 472 (1981).
[CrossRef]

V. N. Bagratashvili, V. S. Letokhov, A. A. Makarov, E. A. Ryabov, Multiple-Photon Processes in Molecules under IR Laser Radiation (Viniti, Moscow, 1981).

Sarishvili, O. G.

O. G. Sarishvili et al., At. Energ. 43, 210 (1977).
[CrossRef]

Willis, C.

M. Gauthier, W. S. Nip, P. A. Hackett, C. Willis, Chem. Phys. Lett. 69, 372 (1980).
[CrossRef]

At. Energ.

O. G. Sarishvili et al., At. Energ. 43, 210 (1977).
[CrossRef]

Chem. Phys. Lett.

M. Gauthier, W. S. Nip, P. A. Hackett, C. Willis, Chem. Phys. Lett. 69, 372 (1980).
[CrossRef]

V. S. Doljikov, V. R. Kolomisky, E. A. Ryabov, Chem. Phys. Lett. 80, 472 (1981).
[CrossRef]

Kvantovaya Elektron. (Moscow)

V. Yu. Baranov et al., Kvantovaya Elektron. (Moscow) 6, 811 (1979) [Sov. J. Quantum. Electron. 9, 480 (1979)].

G. I. Abdushelishvili et al., Kvantovaya Elektron. (Moscow) 8, 534 (1981) [Sov. J. Quantum Electron. 12, 459 (1982)].

Pis’ma Zh. Eksp. Teor. Fiz.

R. V. Ambartsumian et al., Pis’ma Zh. Eksp. Teor. Fiz. 20, 597 (1974) [JETP Lett. 20, 273 (1974)].

Pis’ma Zh. Tekh. Fiz.

G. I. Abdushelishvili et al., Pis’ma Zh. Tekh. Fiz. 5, 14849 (1979) [Sov. Tech. Phys. Lett. 5, 350 (1979)].

Usp. Fiz. Nauk

N. V. Karlov, A. M. Prokhorov, Usp. Fiz. Nauk 118, 583 (1976) [Sov. Phys. Usp. 19, 285 (1976)].
[CrossRef]

Other

V. S. Letokhov, C. B. Moore, Chemical and Biochemical Applications of Lasers, C. B. Moore, Ed. (Academic, New York, 1977), Vol. 3, p. 1.

V. N. Bagratashvili, V. S. Letokhov, A. A. Makarov, E. A. Ryabov, Multiple-Photon Processes in Molecules under IR Laser Radiation (Viniti, Moscow, 1981).

I. G. Gverdtsiteli, E. D. Oziashvili, Production of Isotopes (Atomizdat, Moscow, 1973).

G. I. Abdushelishvili et al., in Proceedings, Fourth International Symposium on Gas Flow and Chemical Lasers, Stresa, 1982.

A. B. Bakhatdze, Stable Isotopes in the Life Sciences (International Atomic Energy Agency, Vienna, 1977).

K. Cohen, The Theory of Isotope Separation (McGraw-Hill, New York, 1951).

O. N. Avatokov et al., in Proceedings, Eleventh Conference on Coherent and Nonlinear Optics, Erevan, 1982, p. 672.

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Figures (7)

Fig. 1
Fig. 1

Schematic of the isotope separation process.

Fig. 2
Fig. 2

Carbon-13 concentration dependence on the number of cycles.

Fig. 3
Fig. 3

Carbon-13 dissociation yield dependence on the total pressure of the absorber and buffer or scavenger gases.

Fig. 4
Fig. 4

Selectivity dependence on the pressure of the absorber gas for the different CO2 laser emission lines.

Fig. 5
Fig. 5

Selectivity dependence on the total pressure of the absorber and buffer gases for the different CO2 laser emission lines.

Fig. 6
Fig. 6

Carbon-13 dissociation yield dependence on the pressure of the absorber gas for the different CO2 laser emission lines.

Fig. 7
Fig. 7

Carbon-13 dissociation yield dependence on the total pressure of the absorber and buffer gases for the different CO2 laser emission lines.

Tables (1)

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Table I Selectivity and Dissociation Yield Values for a Single-Pulse Regime

Equations (1)

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L P = x p - x 0 x 0 ( 1 - x 0 ) ( α - 1 ) ,

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