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Tracking Electronic and Molecular Structural Dynamics during Dissociation of the Photocatalyst Mn2(CO)10 via Time-Resolved X-Ray Spectroscopy

Hana Cho, Kiryong Hong, Mathew L. Strader, Jae Hyuk Lee, Robert W. Schoenlein, Nils Huse, and Tae Kyu Kim

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Abstract

The molecular structure dynamics and transient valence charge distribution during the photo-dissociation of the photocatalyst Mn2(CO)10 are revealed via time-resolved x-ray spectroscopy at the Mn K-edge, combined with quantum chemistry simulations.

© 2014 Optical Society of America

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