Atomic Rydberg-state spectroscopy of Ca i using pulsed color-center lasers

R. Beigang; J. J. Wynne

doi:10.1364/OL.6.000295

Optics Letters
Vol. 6,
Issue 6,
pp. 295-297
(1981)
•https://doi.org/10.1364/OL.6.000295

Atomic Rydberg-state spectroscopy of Ca i using pulsed color-center lasers

R. Beigang and J. J. Wynne

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R. Beigang and J. J. Wynne, "Atomic Rydberg-state spectroscopy of Ca i using pulsed color-center lasers," Opt. Lett. 6, 295-297 (1981)

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Abstract

The utility of using color-center lasers for atomic spectroscopy is demonstrated. Pulsed, color-center lasers are used in conjunction with pulsed dye lasers for multiphoton ionization spectroscopy studies of Ca i. The $4 s 6 d^{1} D_{2} - 4 snf^{1} F_{3}^{°}$ spectrum for n = 11–16 is observed. Two other series of lines are identified as $4 s 5 f^{1} F_{3}^{°} - 4 sng^{1} G_{4}$ and X–4sng ¹G₄ transitions.

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	$4 s 6 d^{1} D_{2} - 4 snf^{1} F_{3}^{°}$ Transitions
n	ν_CCL (cm⁻¹)	$E_{4 s 6 d^{1} D_{2}} + ν_{CCL} ({cm}^{- 1})$	$E_{4 sn f^{1} F_{3}^{°}} ({cm}^{- 1})$
11	3394.3 ± 0.2	48384.1 ±0.2	48384.04^a
12	3541.9 ± 0.2	48531.7 ± 0.2	48532.14^a
13	3657.6 ± 0.2	48647.4 ± 0.2	48647.30^b
14	3748.7 ± 0.2	48738.5 ± 0.2	48738.54^b
15	3822.3 ± 0.2	48812.1 ± 0.2	48812.09^b
16	3881 ± 1	48871 ± 1	48872.20^b

$4 s 5 f^{1} F_{3}^{°} - 4 sng^{1} G_{4}$ Transitions
Label	ν_CCL (cm⁻¹)	n	$E_{4 sn g^{1} G_{4}} = E_{4 s 5 f^{1} F_{3}^{°}} + ν_{CCL} ({cm}^{- 1})$	n^*
A₁	3397.3 ± 0.3	10	48202.2 ± 0.3	9.971
A₂	3589.4 ± 0.5	11	48394.3 ± 0.5	10.971
A₃	3735.2 ± 0.2	12	48540.1 ± 0.2	11.970
A₄	3848.8 ± 0.3	13	48653.7 ± 0.3	12.970
	X–4sng ¹G₄ Transitions
Label	ν_CCL (cm⁻¹)	n	$E_{4 sn g^{1} G_{4}} = E_{X} + ν_{CCL} ({cm}^{- 1})$	n^*

B₁	3332 ± 1	10	48204	9.979
B₂	3522.6 ± 0.2	11	48394.6	10.973
B₃	3668.2 ± 0.2	12	48540.2	11.971
B₄	3781.1 ± 0.2	13	48653.1	12.964
B₅	3871.4 ± 0.6	14	48743.4	13.966

	$4 s 6 d^{1} D_{2} - 4 snf^{1} F_{3}^{°}$ Transitions
n	ν_CCL (cm⁻¹)	$E_{4 s 6 d^{1} D_{2}} + ν_{CCL} ({cm}^{- 1})$	$E_{4 sn f^{1} F_{3}^{°}} ({cm}^{- 1})$
11	3394.3 ± 0.2	48384.1 ±0.2	48384.04^a
12	3541.9 ± 0.2	48531.7 ± 0.2	48532.14^a
13	3657.6 ± 0.2	48647.4 ± 0.2	48647.30^b
14	3748.7 ± 0.2	48738.5 ± 0.2	48738.54^b
15	3822.3 ± 0.2	48812.1 ± 0.2	48812.09^b
16	3881 ± 1	48871 ± 1	48872.20^b

$4 s 5 f^{1} F_{3}^{°} - 4 sng^{1} G_{4}$ Transitions
Label	ν_CCL (cm⁻¹)	n	$E_{4 sn g^{1} G_{4}} = E_{4 s 5 f^{1} F_{3}^{°}} + ν_{CCL} ({cm}^{- 1})$	n^*
A₁	3397.3 ± 0.3	10	48202.2 ± 0.3	9.971
A₂	3589.4 ± 0.5	11	48394.3 ± 0.5	10.971
A₃	3735.2 ± 0.2	12	48540.1 ± 0.2	11.970
A₄	3848.8 ± 0.3	13	48653.7 ± 0.3	12.970
	X–4sng ¹G₄ Transitions
Label	ν_CCL (cm⁻¹)	n	$E_{4 sn g^{1} G_{4}} = E_{X} + ν_{CCL} ({cm}^{- 1})$	n^*

B₁	3332 ± 1	10	48204	9.979
B₂	3522.6 ± 0.2	11	48394.6	10.973
B₃	3668.2 ± 0.2	12	48540.2	11.971
B₄	3781.1 ± 0.2	13	48653.1	12.964
B₅	3871.4 ± 0.6	14	48743.4	13.966

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