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Ultrafast Spatial Dynamics of Excitons During Intramolecular Singlet Fission

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Abstract

Using ultrafast transient absorption and emission spectroscopy, we probe the spatial dynamics of excitons during intramolecular singlet fission in asymmetric oligoacene heterodimers. Exciton-exciton correlations are crucial for promoting both triplet pair formation and recombination.

© 2016 Optical Society of America

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