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Conferences > UP > 2016 > UTu4A > UTu4A.15

Ultrafast Vibrational Spectroscopy Reveals the Primary Photochemical Processes of a Ferracyclobutadiene

Boris Wezisla, Joel Torres-Alacan, Ujjal Das, Jörg Lindner, Alexander C. Filippou, and Peter Vöhringer

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Abstract

The primary photoinduced processes of distorted square-pyramidal ferracyclobutadiene tricarbonyl have been studied in liquid acetonitrile solution under ambient conditions using femtosecond UV-pump mid-infrared-probe spectroscopy. The dynamics are governed by the dissociation of an equatorial CO ligand on a time scales of a few picoseconds followed by the filling of the resultant vacancy by a solvent molecule.

© 2016 Optical Society of America

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