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Electronic Dynamics in Highly Excited States of Acetone and Methyl Azide Studied with Ultrafast PEPICO Spectroscopy

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Abstract

Excited electronic states near 8.0 eV are studied using femtosecond PEPICO spectroscopy, accessing dense manifolds of strongly coupled states. Ionization to multiple cation states is crucial for navigating the mixed states of this energy regime.

© 2016 Optical Society of America

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