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Coherent Wavepacket Evolution Analysis Reveals a Conical Intersection in a Highly Fluorescent Molecule

Johanna Brazard, Laurie A. Bizimana, William P. Carbery, Tobias Gellen, and Daniel B. Turner

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Abstract

Time−frequency analysis of high-sensitivity transient absorption spectra acquired using sub-8 fs laser pulses reveals phase shifts of the coherent wavepacket evolution signal due to the unexpected propagation of a wavepacket through a conical intersection.

© 2016 Optical Society of America

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