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Coherent Two-Dimensional Spectroscopy of Exciton-Exciton Interactions

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Abstract

We theoretically show that exciton-exciton interaction in molecular systems can be directly monitored by fifth-order non-linear optical signals of -2k1+2k2+k3 type. The concept is experimentally demonstrated on exciton-exciton annihilation in perylene bisimide aggregates.

© 2016 Optical Society of America

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