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Coherence Between Energetically-Remote Chromophores in a Marine Algae Antenna Complex

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Abstract

Two-dimensional electronic spectroscopy and broadband transient absorption were executed over the full spectrum of phycocyanin 645 (PC645, Chroomonas mesostigmatica) at 295 and 77 K to reveal vibronic coherence between donor/acceptors separated by >1500 cm−1.

© 2016 Optical Society of America

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