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Studying Spatio-Energetic Dynamics in Light Harvesting Complex II using Two-Dimensional Electronic-Vibrational Spectroscopy

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Abstract

We present two-dimensional electronic-vibrational spectra of the chlorophyll (Chl) binding protein light harvesting complex II (LHCII) from spinach, and of isolated Chl a and Chl b. We show how energy transfer from Chl b to Chl a and subsequent relaxation can be directly observed in LHCII using this multidimensional technique.

© 2016 Optical Society of America

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