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Synchrotron and X-Ray Free Electron Laser Studies of High-Valent Iron Formation with X-ray Absorption Spectroscopy

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Abstract

Ultrafast X-ray techniques serve as a direct probe of a long-lived pseudo-octahedral high-valent iron(V) complex. Its photo-induced formation from an azido-iron(III) precursor is observed in real-time with sub-picosecond resolution at SACLA XFEL.

© 2016 Optical Society of America

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