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Hydrogen Bond Enhancement of Fermi Resonances Explored with Ultrafast IR Two-Colour Pump-Probe and 2D-IR Spectroscopy

Christian Greve, Rene Costard, Henk Fidder, and Erik T.J. Nibbering

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Abstract

Ultrafast polarisation-resolved 2D-IR mapping the fundamental and first overtone N-H stretching manifolds, and two-colour IR pump-probe experiments following transient population dynamics characterize a key role of a Fermi resonance with the NH2-bending in aniline-dimethylsulfoxide complexes.

© 2014 Optical Society of America

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