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Ultrafast Interaction of Dark and Bright Electronic States in Open-Chain Carotenoids Investigated by Pump-DFWM

T. Miki, T. Buckup, M. Marek, R. J. Cogdell, and M. Motzkus

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Abstract

Coupling between dark and bright electronic states in carotenoids was observed in the ultrafast evolution of vibrational coherence and in the non-oscillatory signal of pump-DFWM. Coupling efficiency depends on the number of conjugated double bonds.

© 2014 Optical Society of America

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