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Spontaneous formation of correlated charge coherence induced by 1.5-cycle pulse in 1-D organic metal (TMTTF)2AsF6

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Abstract

Ultrafast optical response of organic metal (TMTTF)2AsF6 induced by 1.5 cycle (7 fs) infrared pulse was investigated. Intense coherent oscillation of correlated charge (18 fs) grows in the time scale of 50 fs, reflecting the spontaneous-formation of the electronic coherence before the electronic thermalization.

© 2014 Optical Society of America

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