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Vibrational Dynamics of the CN Stretching in the Electronically Excited State by UV and Visible-Pump and Infrared-Probe Spectroscopy

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Abstract

We have carried out visible-pump infrared-probe measurements on a CN-containing coumarin in a protic solvent. The time-dependent changes of the infrared spectra are measured on a picoseconds time scale, likely because of vibrational cooling.

© 2014 Optical Society of America

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