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Ultrafast Vibrational Dynamics in Quasi-Linear Arrays of Hydrogen-Bonds Explored by 2DIR-Spectroscopy

Stephan Knop, Jaane Seehusen, Jörg Lindner, Dirk Schwarzer, and Peter Vöhringer

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Abstract

Femtosecond mid-infrared pump-probe and two-dimensional spectroscopy in the OH-stretching spectral region was used to elucidate the dynamics of vibrational energy relaxation and dynamic line broadening in artificial low-dimensional hydrogen-bond wires of different lengths.

© 2010 Optical Society of America

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