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Non-Born-Oppenheimer wavepacket revivals in a polyatomic molecule

A. E. Boguslavskiy, D. Townsend, M. S. Schuurman, and A. Stolow

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Abstract

Non-Born-Oppenheimer wavepacket revivals have been observed in 1,4-diazabicyclo[2.2.2]octane using time resolved photoelectron spectroscopy. Upon photoexcitation, the wavepacket oscillates between the first two excited states for over 14 ps – a behavior only seen in diatomics before.

© 2010 Optical Society of America

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