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Time-Energy Map of Photoelectron Angular Anisotropy for Investigation of Ultrafast Internal Conversion

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Abstract

Ultrafast internal conversion of pyrazine through a conical intersection was observed by photoelectron imaging with 22 fs time-resolution. The 2D time-energy map of the photoelectron angular anisotropy revealed a clear signature of the internal conversion.

© 2010 Optical Society of America

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