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Monitoring the External Vibrational Control of Excitation-Energy Transfer Using Pump-Probe Polarization Spectroscopy

Jason D. Biggs and Jeffrey A. Cina

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Abstract

We have developed a method for controlling electronic-excitation transfer in chromophore dimers using pulse-induced nuclear motion. We further developed the framework needed to simulate various nonlinear optical experiments on such systems.

© 2010 Optical Society of America

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