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Uncovering Coherent and Incoherent Vibrational Interactions in a Transition Metal Mixed Valence Complex Using Femtosecond Two-Dimensional Infrared Spectroscopy

Michael S. Lynch, Mark Cheng, Benjamin E. Van Kuiken, Stephanie Daifuku, and Munira Khalil

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Abstract

Femtosecond polarization-selective nonlinear infrared spectroscopies reveal a detailed molecular picture of coherent and incoherent vibrational relaxation dynamics of a cyano-bridged mixed valence complex in a polar solvent.

© 2010 Optical Society of America

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