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Highly efficient energy transfer in a dyad with orthogonally arranged transition dipole moments: Beyond the Limits of Förster?

Igor Pugliesi, Andreas Walter, Heinz Langhals, and Eberhard Riedle

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Abstract

Perylene bisimide dyads mediate an ultrafast energy transfer contradicting the Förster approximation through their transition densities. The high monomeric fluorescence quantum yield leads to near unit efficiency making them suitable candidates for molecular electronic circuitry.

© 2010 Optical Society of America

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