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Two-Dimensional Electronic Spectroscopy of Semiconducting Single-Walled Carbon Nanotubes

Matthew W. Graham, Tessa R. Calhoun, Alex A. Green, Mark C. Hersam, and Graham R. Fleming

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Abstract

Application of 2D Fourier transform electronic spectroscopy to semiconducting SWNTs is demonstrated to decongest complex exciton dynamics. Analysis provides the E22 homogeneous linewidth, and elucidates the roles of vibrational and multi-exciton states in population relaxation.

© 2010 Optical Society of America

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