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Unique Behavior of Lattice Modulation Phase Induced by Ligand Motion of a Mixed-Valence Metal-Halogen Complex

F. Araoka and T. Kobayashi

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Abstract

A highly time-resolved pump-probe measurement for a halogen-bridged mixed-valence metal complex, [Pt(en)2][Pt(en)2Br2](ClO4)4, shows sinusoidal modulations accompanying with a unique behavior of probe-wavelength-dependent phase, suggesting an existence of a ligand motion coupled with the lattice vibration.

© 2006 Optical Society of America

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