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A Femtosecond IR and Raman Look on a Nucleophilic Addition in the Electronic Ground State

S. Laimgruber, H. Schachenmayr, W. Schreier, and P. Gilch

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Abstract

A highly reactive ketene intermediate is formed in its electronic ground state via photo-induced hydrogen transfer in 400 fs. The mechanistic details of a nucleophilic addition to this ketene are revealed by femtosecond vibrational spectroscopy.

© 2006 Optical Society of America

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