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Ultrafast Chelation Dynamics of Model Photoswitches: Cyclopentadienyl Manganese and Arene Chromium Tricarbonyl Derivatives with Pendant Sulfides

Tung T. To, Edwin J. Heilweil, Charles B. Duke, and Theodore J. Burkey

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Abstract

The chelation dynamics of [Mn{η5-C5H4C(O)R}(CO)3] and [Cr{η6-C6H5C(O)R}(CO)3] (R=CH2(SCH3), CH(SCH3)2, C(SCH3)3) in solution were investigated on the picosecond timescale. Tailoring the side chain structure and solvent environment influences the reaction rates and chelation pathways.

© 2006 Optical Society of America

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