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2D optical spectroscopy of a conjugated polymer with tunable visible 15 fs-pulses from a 200 kHz NOPA

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Abstract

We investigate inter-site electronic coupling and ultrafast dynamics of delocalized molecular excitons in a conjugated polymer by two-dimensional heterodyned three-pulse photon echoes. This gives unbiased insight into exciton scattering and the time-evolution of electron-phonon coupling.

© 2006 Optical Society of America

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