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Observation of Anharmonic Coupling in the Time Domain with Femtosecond Stimulated Raman

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Abstract

Coherent motion of low frequency bending vibrations is impulsively excited in CDCl3 and subsequent couplings between the C-D stretch and the low frequency coherences are detected in real time by femtosecond stimulated Raman spectroscopy (FSRS).

© 2006 Optical Society of America

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