Vibrational energy relaxation in water-acetonitrile mixtures

Dan Cringus; Sergey Yeremenko; Maxim S. Pshenichnikov; Douwe A. Wiersma

14th International Conference on Ultrafast Phenomena
Technical Digest (CD) (Optica Publishing Group, 2004),
paper MB5

Vibrational energy relaxation in water-acetonitrile mixtures

Dan Cringus, Sergey Yeremenko, Maxim S. Pshenichnikov, and Douwe A. Wiersma

International Conference on Ultrafast Phenomena 2004

Niigata Japan
25–30 July 2004
ISBN: 3-54024-110-8

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Hydrogen Bond Dynamics (MB)

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D. Cringus, S. Yeremenko, M. S. Pshenichnikov, and D. A. Wiersma, "Vibrational energy relaxation in water-acetonitrile mixtures," in 14th International Conference on Ultrafast Phenomena, Technical Digest (CD) (Optica Publishing Group, 2004), paper MB5.

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Abstract

IR pump-probe spectroscopy is used to study the effect of hydrogen bonding on the vibrational energy relaxation pathways. Hydrogen bonding accelerates the population relaxation from 12ps in diluted acetonitrile solution to 700fs in bulk water.

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