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Observation of Frequency-Dependent Friction During Barrierless Photo-Isomerization of 1,1’-Diethyl-2,2’-Cyanine Iodide in n-Alcohol Solutions

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Abstract

Having resolved the entire downhill motion of the excited state population during photo-induced isomerization we have recorded a clear difference in viscosity dependence of lifetime of reaction transients on their location on excited state potential.

© 2000 Optical Society of America

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