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Conferences > QELS > 2012 > QM2G > QM2G.5

Quantum coherence controls the charge separation in a prototypical artificial light harvesting system

S. M. Falke, C. A. Rozzi, N. Spallanzani, A. Rubio, E. Molinari, D. Brida, M. Maiuri, G. Cerullo, H. Schramm, J. Christoffers, and C. Lienau

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Abstract

Ultrafast spectroscopy and quantum-dynamics simulations of an artificial supramolecular light-harvesting system give strong evidence that the quantum-correlated wavelike motion of electrons and nuclei governs the ultrafast electronic charge transfer.

© 2012 Optical Society of America

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