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Conferences > QELS > 2001 > QME > QME4
  • Quantum Electronics and Laser Science Conference
  • OSA Technical Digest (Optica Publishing Group, 2001),
  • paper QME4

Nonlocal effects in the nonlinear optical response of chiral molecules: Third-order nonlinear circular dichroism

H. Mesnil, M. C. Schanne-Klein, and F. Hache

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Abstract

Although it was predicted as soon as 1967,1 third- order nonlinear circular dichroism has never been experimentally observed. In this paper, we investigate this phenomenon in a liquid of chiral molecules. We first perform a theoretical calculation including nonlocal effects in the nonlinear light-matter interaction that allows to get insight into the process and to obtain its order of magnitude.2

© 2001 Optical Society of America

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