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Conferences > QELS > 1995 > QWE > QWE2
  • Quantum Electronics and Laser Science Conference
  • OSA Technical Digest (Optica Publishing Group, 1995),
  • paper QWE2

Femtosecond hyper-Rayleigh scattering of spatial-orientational correlations between chromophores

Koen Clays, Marvin Wu, and André Persoons

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Abstract

Hyper-Rayleigh scattering (HRS) has been used to probe the spatial-orientational distribution function of nonlinear optical chromophores in the solid state. The fluctuations in this function cause a hyper-Rayleigh scattering signal that fluctuates as a function of position. The decay of the autocorrelation function of this fluctuating signal is characterized by a spatial correlation length. This length indicates the degree of spatial correlation between the chromophores.

© 1995 Optical Society of America

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