Terahertz time-domain spectroscopy of methyl chloride vapor

H. Harde; N. Katzenellenbogen; N. Katzenellenbogen; D Grischkowsky; D Grischkowsky

Quantum Electronics and Laser Science Conference
OSA Technical Digest (Optica Publishing Group, 1993),
paper QTuJ4

Terahertz time-domain spectroscopy of methyl chloride vapor

H. Harde, N. Katzenellenbogen, and D Grischkowsky

Quantum Electronics and Laser Science Conference 1993

Baltimore, Maryland United States
2–7 May 1993
ISBN: 1-55752-302-9

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Molecular Spectroscopy (QTuJ)

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H. Harde, N. Katzenellenbogen, and D. Grischkowsky, "Terahertz time-domain spectroscopy of methyl chloride vapor," in Quantum Electronics and Laser Science Conference, D. Auston, D. Steel, T. Heinz, and G. Stegeman, eds., Vol. 12 of OSA Technical Digest (Optica Publishing Group, 1993), paper QTuJ4.

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Abstract

By using the newly developed optoelectronic terahertz beam system^1,2 shown in Fig. 1(a), the propagation of femtosecond terahertz pulses through spectrally dense methyl chloride vapor was investigated. Our observations indicate that the individual rotational transitions have van Vleck-Weiss-kopf line shapes, with a strong nonmonotonic dependence for the collisionbroadening coefficient.

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