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Conferences > QELS > 1993 > QTuI > QTuI2
  • Quantum Electronics and Laser Science Conference
  • OSA Technical Digest (Optica Publishing Group, 1993),
  • paper QTuI2

Intermolecular vibrations in liquids: anisotropic librational dynamics in substituted benzenes

Dale McMorrow, Joseph S. Melinger, and William T. Lotshaw

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Abstract

Femtosecond nonlinear-optical (NLO) spectroscopies exhibit significant advantages over spontaneous scattering techniques for probing the Rayleigh-wing region of the light-scattering (LS) spectra of liquids. Because of the intense central Lorentzian feature present in the LS spectra of liquids, the extraction of detailed dynamical information on low-frequency intermolecular vibrational resonances has proven difficult. We report here the results of an extensive investigation into the dynamics of intermolecular vibrations in liquids.

© 1993 Optical Society of America

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