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Spectral Oscillation in Chlorophyll a Revealed by Ultrafast Real-time Vibrational Spectroscopy

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Abstract

Broadband real-time vibrational spectroscopy was used to investigate the vibronic dynamics in Chl-a for the first time. Spectral distribution of the vibrational amplitudes was observed and interpreted as energy exchange intermediated by vibrational coherence.

© 2011 Optical Society of America

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