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Coherent Control of Fluorescence Intensity with Shaped Femtosecond Pulses in Organic Molecules

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Abstract

This paper presents a study of the coherent control of fluorescence intensity by two- photon absorption via genetic algorithm in Y-shaped molecules. Using a spatial light modulator, we were able to enhance the fluorescence intensity of two of these molecules. We also measured the two-photon absorption spectra to understand the different behavior of the two molecules.

© 2009 Optical Society of America

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