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Third Harmonic Generation of Vanadyl-Phthalocyanine Film Prepared on NaCl Substrate by Molecular Beam Epitaxy

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Abstract

The incident angle dependence of TH intensity of VOPc film irradiated with P polarized laser beam shows an upper convex curve that has a maximum value at −15 degree. It suggest that the tensor of TH susceptibility of VOPc film is dominated with the components of χ(xxxx) and χ(yyyy) and also indicates that the VOPc molecules deposited on NaCl have a tilt angle. These may give us information about THG.

© 2000 Optical Society of America

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