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Time-Resolved High-Harmonic Spectroscopy of Photochemical Dynamics

H. J. Wörner, J. B. Bertrand, P. B. Corkum, and D. M. Villeneuve

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Abstract

We use high-harmonic spectroscopy to observe the evolution of the electronic structure of molecules undergoing an ultrafast photochemical reaction. Using the transient grating technique allows us to determine amplitude and phase of the excited state emission.

© 2010 Optical Society of America

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